Recently, digital gamma-ray spectroscopy employing low-cost and publicly available (Commercial off the shelf) digitizers has been frequently used in different studies worldwide. In this paper, we considered the digital methods for gamma-ray spectroscopy in which the anode pulses of the photomultiplier tube (PMT) output in a NaI(Tl) scintillation detector were immediately digitized by a PC sound card. We introduced and developed the methods for gamma-ray spectroscopy of microCurie gamma-ray sources by a sampling rate of 96 kHz. First, at low count rates, the pulse arrival time was determined directly by the raw waveform, and the gamma-ray spectrum was obtained by summing the corresponding values in the samples per pulse. In addition, the gamma-ray spectrum was obtained by an enhanced sampling rate waveform and the pulse arrival time was determined by employing the digital constant fraction discrimination (DCFD) method, where each pulse area was achievable by summing the corresponding values of pulse samples. On the other hand, fitting the appropriate model function on the pulses and obtaining the fitted pulse area were undertaken for gamma-ray spectroscopy. To this end, a non-iterative algorithm to fast fit the Gaussian model function was improved. Moreover, the pile-up correction was performed at different count rates employing the Maximum Likelihood Estimation (MLE) method and Gaussian model function. Also, an approximate method for solving the high run time challenge was identified in the MLE method for long-time waveforms. To reject the pile-up events, a method was introduced based on the calculation of the full-width at half maximum pulses. By applying the proposed rejection method, we achieved an energy resolution of 6.2% at 663 keV gamma-rays and a count rate of 5.3 kcps.
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http://dx.doi.org/10.1016/j.apradiso.2021.109854 | DOI Listing |
Exp Astron (Dordr)
January 2025
Space Sciences Laboratory, University of California, Berkeley, 7 Gauss Way, Berkeley, 94720 CA USA.
We present an investigation into the effects of high-energy proton damage on charge trapping in germanium cross-strip detectors with the goal of accomplishing three important measurements. First, we calibrated and characterized the spectral resolution of a spare COSI-balloon detector in order to determine the effects of intrinsic trapping, finding that electron trapping due to impurities dominates over hole trapping in the undamaged detector. Second, we performed two rounds of proton irradiation of the detector in order to quantify, for the first time, the rate at which charge traps are produced by proton irradiation.
View Article and Find Full Text PDFJ Am Chem Soc
January 2025
Department of Physics, Alba Nova Research Center, Stockholm University, Stockholm SE-106 91 Sweden.
Iron-doped nickel oxyhydroxides, Ni(Fe)OH, are among the most promising oxygen evolution reaction (OER) electrocatalysts in alkaline environments. Although iron (Fe) significantly enhances the catalytic activity, there is still no clear consensus on whether Fe directly participates in the reaction or merely acts as a promoter. To elucidate the Fe's role, we performed X-ray spectroscopy studies supported by DFT on Ni(Fe)OH electrocatalysts.
View Article and Find Full Text PDFSci Rep
January 2025
Depto de Química, Universidade Federal de Minas Gerais, Belo Horizonte, MG, CEP 31.270-901, Brazil.
Magnetoliposomes containing magnetite, soy lecithin, stigmasterol, and beta-sitosterol of the mean size minor than 160 nm were obtained by a scalable and green process using autoclave and sonication without organic solvents. The formation, size of the liposome, linkage, and encapsulation of the magnetite were evaluated by Cryo-TEM. The stability of magnetoliposomes after storage for 6 months at 4 °C was improved by liposome size, the ability of soy lecithin to preserve the magnetite phase against oxidation, pH, polydispersity index, and zeta potential.
View Article and Find Full Text PDFAppl Microbiol Biotechnol
January 2025
Key Laboratory of Medical Molecule Science and Pharmaceutics Engineering, Ministry of Industry and Information Technology, Institute of Biochemical Engineering, School of Chemistry and Chemical Engineering, Beijing Institute of Technology, Beijing, 100081, China.
Butenyl-spinosyn, derived from Saccharopolyspora pogona, is a broad-spectrum and effective bioinsecticide. However, the regulatory mechanism affecting butenyl-spinosyn synthesis has not been fully elucidated, which hindered the improvement of production. Here, a high-production strain S.
View Article and Find Full Text PDFHeliyon
January 2025
Department of Physics, College of Science, De La Salle University, Philippines.
Exposure to mid-energy radiation poses significant health risks, necessitating the development of effective shielding materials. Traditional lead-based shields, while effective, have significant drawbacks including toxicity and environmental concerns. This study investigates the potential of lead-free epoxy resin nanocomposites, incorporating bismuth oxide, nickel oxide, and cerium oxide, for mid-energy radiation protection.
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