We report low-temperature muon spin relaxation/rotation (SR) measurements on single crystals of the actinide superconductor UTe. Below 5 K we observe a continuous slowing down of magnetic fluctuations that persists through the superconducting transition temperature ( = 1.6 K), but we find no evidence of long-range or local magnetic order down to 0.025 K. The temperature dependence of the dynamic relaxation rate down to 0.4 K agrees with the self-consistent renormalization theory of spin fluctuations for a three-dimensional weak itinerant ferromagnetic metal. Our SR measurements also indicate that the superconductivity coexists with the magnetic fluctuations.
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http://dx.doi.org/10.1103/physrevb.100.140502 | DOI Listing |
Sci Rep
January 2025
Water Management Research Institute, National Water Research Center, Shubra El-Kheima 13411, Cairo, Egypt.
The exploration of perovskite compounds incorporating actinide and divalent elements reveals remarkable characteristics. Focusing on PbBkO, RaBkO, and SrBkO, these materials were studied using density functional theory (DFT) via the CASTEP code to analyze their electronic, optical, and mechanical properties. The results show semiconductor behavior, with respective band gaps of 1.
View Article and Find Full Text PDFJ Phys Condens Matter
January 2024
School of Physical Science and Technology, ShanghaiTech University, Shanghai 201210, People's Republic of China.
The research on hydrogen-rich ternary compounds attract tremendous attention for it paves new route to room-temperature superconductivity at lower pressures. Here, we study the crystal structures, electronic structures, and superconducting properties of the ternary Ca-U-H system, combining crystal structure predictions withcalculations under high pressure. We found four dynamically stable structures with hydrogen clathrate cages: CaUH-, CaUH--3, CaUH--31, and CaUH--3.
View Article and Find Full Text PDFSci Rep
October 2023
Department of Physics, University of Central Florida, Orlando, FL 32816 USA.
Charge density wave (CDW) ordering has been an important topic of study for a long time owing to its connection with other exotic phases such as superconductivity and magnetism. The [Formula: see text] (R = rare-earth elements) family of materials provides a fertile ground to study the dynamics of CDW in van der Waals layered materials, and the presence of magnetism in these materials allows to explore the interplay among CDW and long range magnetic ordering. Here, we have carried out a high-resolution angle-resolved photoemission spectroscopy (ARPES) study of a CDW material [Formula: see text], which is antiferromagnetic below [Formula: see text], along with thermodynamic, electrical transport, magnetic, and Raman measurements.
View Article and Find Full Text PDFRep Prog Phys
April 2023
Institute of Physics (FZU), Czech Academy of Sciences, Na Slovance 2,182 00 Prague, Czech Republic.
Hydrides of actinides, their magnetic, electronic, transport, and thermodynamic properties are discussed within a general framework of H impact on bonding, characterized by volume expansion, affecting mainly the 5states, and a charge transfer towards H, which influences mostly the 6and 7states. These general mechanisms have diverse impact on individual actinides, depending on the degree of localization of their 5states. Hydrogenation of uranium yields UHand UH, binary hydrides that are strongly magnetic due to the 5band narrowing and reduction of the 5-6hybridization.
View Article and Find Full Text PDFJ Am Chem Soc
July 2022
State Key Laboratory of Superhard Materials and International Center for Computational Method & Software, College of Physics, Jilin University, Changchun 130012, China.
Achieving room-temperature superconductivity has been an enduring scientific pursuit driven by broad fundamental interest and enticing potential applications. The recent discovery of high-pressure clathrate superhydride LaH with superconducting critical temperatures () of 250-260 K made it tantalizingly close to realizing this long-sought goal. Here, we report a remarkable finding based on an advanced crystal structure search method of a new class of extremely hydrogen-rich clathrate superhydride MH (M: rare-earth/actinide atom) stoichiometric compounds stabilized at an experimentally accessible pressure of 350 GPa.
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