Variations of bioaerosol characteristics during the process of haze pollution have rarely been explored. In this study, high time-resolved variations of the community structures of bacteria, fungi, and ammonia-oxidizing microorganisms (AOMs) were assessed during a typical haze pollution process. The impacts of meteorological factors, water-soluble inorganic ions (WSII), and organic dicarboxylic acids (DCA) on the airborne microbial community were systematically evaluated. The results showed that the bacterial community varied greatly during the formation stages of haze pollution, and tended to stabilize with the further development of haze pollution. Nevertheless, variations of the fungal community lasted throughout the whole haze pollution process. Furthermore, Nitrososphaera absolutely dominated the ammonia-oxidizing archaea (AOA) and declined as PM burst. Network analysis identified relatively weak interactions and co-occurrence patterns between dominant fungal genera. Importantly, dust source ions and PM acidity exerted the most significant impacts on bacterial and fungal communities. These results identify the high time-resolved variations of airborne microbial communities during the formation and development of haze pollution process, and provide valuable data to better understand the interaction between bioaerosols and haze pollution.
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http://dx.doi.org/10.1016/j.jhazmat.2021.125722 | DOI Listing |
Environ Sci Technol
January 2025
Department of Civil and Environmental Engineering, The Hong Kong Polytechnic University, Hong Kong SAR 999077, China.
Chlorine radicals (Cl) are highly reactive and affect the fate of air pollutants. Several field studies in China have revealed elevated levels of daytime molecular chlorine (Cl), which, upon photolysis, release substantial amounts of Cl but are poorly represented in current chemical transport models. Here, we implemented a parametrization for the formation of daytime Cl through the photodissociation of particulate nitrate in acidic environments into a regional model and assessed its impact on coastal air quality during autumn in South China.
View Article and Find Full Text PDFEnviron Sci Technol
January 2025
State Key Joint Laboratory of Environment Simulation and Pollution Control, Research Center for Eco-Environmental Sciences, Chinese Academy of Sciences, Beijing 100085, China.
Ammonia emissions from vehicles and power plants cause severe environmental issues, including haze pollution and nitrogen deposition. Selective catalytic oxidation (SCO) is a promising technology for ammonia abatement, but current catalysts often struggle with insufficient activity and poor nitrogen selectivity, leading to the formation of secondary pollutants. In this study, we developed a bifunctional Ru/Cu-CHA zeolite catalyst for ammonia oxidation, incorporating both SCO sites (Ru) and selective catalytic reduction sites (SCR, Cu).
View Article and Find Full Text PDFRSC Adv
January 2025
Institute of Resources and Environmental Engineering, Shanxi University, Shanxi Yellow River Laboratory Taiyuan China
Coal combustion generates soot-type air pollution, and NO, as a typical pollutant, is the main haze-causing pollutant. The degradation of NO by means of photocatalytic superhydrophobic multifunctional coatings is both durable and economical. The precipitation method was employed to create a p-n type BiOBr/α-FeO photocatalytic binary system.
View Article and Find Full Text PDFEnviron Sci Technol
January 2025
Shanghai Key Laboratory of Atmospheric Particle Pollution and Prevention (LAP3), National Observations and Research Station for Wetland Ecosystems of the Yangtze Estuary, Department of Environmental Science & Engineering, Fudan University, Shanghai 200438, China.
Nitrogen-containing organic compounds (NOCs) in frost serve as a critical pathway for atmospheric nitrogen deposition, significantly impacting the biogeochemical cycles of nitrogen. However, the molecular characteristics of NOCs in frost and their deposition fluxes are scarcely studied. In this work, frost samples, collected in rural Northeast China in the winter of 2023, were analyzed using nontargeted ultrahigh performance liquid chromatography-orbitrap mass spectrometry (UHPLC-Orbitrap MS) to reveal their content in nitrogen-containing organic compounds (NOCs) and explore their wet deposition fluxes.
View Article and Find Full Text PDFEnviron Sci Technol
January 2025
Key Laboratory of Atmospheric Environment and Extreme Meteorology, Institute of Atmospheric Physics, Chinese Academy of Sciences, Beijing 100029, China.
Aerosol ammonium (NH) is a critical component of particulate matter that affects air pollution, climate, and human health. Isotope-based source apportionment of NH is essential for ammonia (NH) mitigation but the role of kinetic vs equilibrium controls on nitrogen isotope (δN) fractionation between NH and NH remains unresolved. Based on concurrent measurements of NH and NH in winter Beijing, we observed that the difference of δN between NH and NH on clean days (3.
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