The route selection of self-propelled filter papers impregnated with camphor for two-branched water channels was investigated. The two-branched water channel was composed of a stem channel and two branch channels, and the branch channels were connected to the stem channel at a junction. When a single camphor paper reached the junction from the stem channel, it selected one of the two routes equivalently. Three or five camphor papers which were placed on a stem channel exhibited either alternate or random route selection depending on the characteristic length between the leading and following papers, . That is, the alternate route selection of the camphor papers for the two-branched water channels was observed at ≤ 25 mm. By contrast, the alternate route selection was broken at > 25 mm. The physicochemical meaning of the threshold value, ∼ 26 mm, between the alternate and random route selections was discussed based on the experimental results. In addition, the distribution length of camphor molecules developed from the leading camphor paper and the change in the spatial gradient of surface tension around the junction supports the value of . These results suggest that autonomous phenomena using inanimate self-propelled objects are important to understand collective motion in living organisms.
Download full-text PDF |
Source |
---|---|
http://dx.doi.org/10.1021/acs.langmuir.1c00644 | DOI Listing |
Phys Chem Chem Phys
January 2025
State Key Laboratory of Green Chemical Engineering and Industrial Catalysis, Center for Computational Chemistry and Research Institute of Industrial Catalysis, School of Chemistry & Molecular Engineering, East China University of Science and Technology, Shanghai 200237, China.
Photoreduction of CO into hydrocarbons is a potential strategy for reducing atmospheric CO and effectively utilizing carbon resources. Cu-deposited TiO photocatalysts stand out in this area due to their good photocatalytic activity and potential methanol selectivity. However, the underlying mechanism and factors controlling product selectivity remain less understood.
View Article and Find Full Text PDFGreen Chem
January 2025
Van't Hoff Institute for Molecular Sciences, University of Amsterdam Science Park 904 1098 XH Amsterdam The Netherlands
The development of sustainable synthetic methods for converting alcohols to amines is of great interest due to their widespread use in pharmaceuticals and fine chemicals. In this work, we present an electrochemical approach by using green electrons for the selective oxidation of benzyl alcohol to benzaldehyde using a NiOOH catalyst, followed by its reductive amination to form benzyl--butylamine. The number of Ni monolayer equivalents on the catalyst was found to significantly influence selectivity, with 2 monolayers achieving up to 90% faradaic efficiency (FE) for benzaldehyde in NaOH, while 10 monolayers performed best in a -butylamine solution (pH 11), yielding 100% FE for benzaldehyde.
View Article and Find Full Text PDFWiley Interdiscip Rev Nanomed Nanobiotechnol
January 2025
School of Pharmacy and Waterloo Institute of Nanotechnology, University of Waterloo, 200 University Avenue West, Waterloo, Ontario, Canada.
Nucleic acid-based vaccines are leading-edge tools in developing next-generation preventative care. Much research has been done to convert vaccine gene therapy from an invasive to a noninvasive administration approach. The lung's large surface area and permeability make the pulmonary route a promising noninvasive delivery option for vaccines, with systemic and local applications.
View Article and Find Full Text PDFNat Commun
January 2025
Zhejiang Key Laboratory of Advanced Fuel Cells and Electrolyzers Technology, Ningbo Institute of Materials Technology and Engineering, Chinese Academy of Sciences, Ningbo, Zhejiang, PR China.
Amine-assisted two-step CO hydrogenation is an efficient route for methanol production. To maximize the overall catalytic performance, both the N-formylation of amine with CO (i.e.
View Article and Find Full Text PDFArch Pediatr
January 2025
Laboratoire de Biomathématiques, Biophysique, Biochimie et Scientométrie (L3BS), Faculté des Sciences de la Nature et de la Vie, Université de Bejaia, 06000 Bejaia, Algérie; Centre de Recherche en Technologies Agro-alimentaires. Route de Targua Ouzemmour, 06000 Bejaia, Algérie.
Objective: Adolescents are meant to spend a large part of their time practicing a hobby or sport, but currently there is a decline in their level of physical activity and sport both inside and outside schools, which can lead to a risk of obesity. The objective of the present study was to examine physical activity in obese adolescents within the school establishments of the province of Bejaia (northeastern Algeria).
Method: To determine the physical activity level (PAL) in the school population, a sample of 3,038 students with obesity comprising 1,635 girls and 1,403 boys was selected.
Enter search terms and have AI summaries delivered each week - change queries or unsubscribe any time!