Disordered dielectrics with structural correlations on length scales comparable to visible light wavelengths exhibit interesting optical properties. Such materials exist in nature, leading to beautiful structural non-iridescent color, and they are also increasingly used as building blocks for optical materials and coatings. In this article, we explore the angular resolved single-scattering properties of micron-sized, disordered colloidal assemblies. The aggregates act as structurally colored supraparticles or as building blocks for macroscopic photonic glasses. We obtain first experimental data for the differential scattering and transport cross-section. Based on existing macroscopic models, we develop a theoretical framework to describe the scattering from densely packed colloidal assemblies on a hierarchy of length scales.

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http://dx.doi.org/10.1364/OE.418735DOI Listing

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