While almost any kind of face mask offers some protection against particles and pathogens of different sizes, the most efficient ones make use of a layered structure where one or more layers are electrically charged. These electret layers are essential for the efficient filtration of difficult-to-capture small particles, yet the exact nature of electrostatic capture with respect to the charge on both the particles and the electret fibres as well as the effect of the immediate environment remain unclear. Here, we explore in detail the electrostatic interactions between the surface of a single charged electret fibre and a model of the SARS-CoV-2 virus. Using Poisson-Boltzmann electrostatics coupled to a detailed spike protein charge regulation model, we show how pH and salt concentration drastically change both the scale and the sign of the interaction. Furthermore, the configuration of the few spike proteins closest to the electret fibre turns out to be as important for the strength of the interaction as their total number on the virus envelope, a direct consequence of spike protein charge regulation. The results of our work elucidate the details of virus electrostatics and contribute to the general understanding of efficient virus filtration mechanisms.
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http://dx.doi.org/10.1039/d1sm00232e | DOI Listing |
RSC Adv
January 2025
State Key Laboratory of Information Photonics and Optical Communications, Beijing University of Posts and Telecommunications Beijing 100876 China
Modification of the dielectric friction layer materials is an ideal way to enhance the output performance of a triboelectric nanogenerator (TENG), but current research mostly focuses on the metal-polymer or metal-SiO materials. In this work, we constructed different TENG models based on polymer C F -SiO electret materials, and the electronic properties of the different contact surfaces were investigated using first principles. We found that the charge transfer in C F -SiO materials occurred only at the contact interface, and it was partially affected by the terminal atoms near the SiO interface.
View Article and Find Full Text PDFNat Commun
January 2025
State Key Laboratory of Advanced Design and Manufacturing Technology for Vehicle, College of Mechanical and Vehicle Engineering, Hunan University, Changsha, China.
Electrostriction is an important electro-mechanical property in poly (vinylidene fluoride) (PVDF) films, which describes the proportional relation between the electro-stimulated deformation and the square of the electric field. Generally, traditional methods to improve the electrostriction of PVDF either sacrifice other crystalline-related key properties or only influence minimal regions around the surface. Here, we design a unique electret structure to fully exploit the benefits of internal crystal in PVDF films.
View Article and Find Full Text PDFMaterials (Basel)
December 2024
Faculty of Chemical and Process Engineering, Warsaw University of Technology, 00-645 Warsaw, Poland.
This study explores the fabrication of electret nonwoven structures for high-efficiency air filtration, utilizing the blow spinning technique. In response to the growing need for effective filtration systems, we aimed to develop biodegradable materials capable of capturing fine particulate matter (PM2.5) without compromising environmental sustainability.
View Article and Find Full Text PDFJ Hazard Mater
December 2024
School of Materials Science and Physics, China University of Mining and Technology, Xuzhou 221116, China; Jiangsu Engineering Research Center of Dust Control and Occupational Protection, Xuzhou 221008, China; College of Polymer Science and Engineering, State Key Laboratory of Polymer Materials Engineering, Chengdu 610065, China. Electronic address:
Particulate matters (PMs), one of the major airborne pollutants, continue to seriously threaten human health and the environment. Here, a self-crystal-induced electret enhancement (SCIEE) strategy was developed to promote the in-situ electret effect and polarization properties of electrospun poly(L-lactic acid) (PLLA) nanofibers. The strategy specifically involved the elaborate pre-structuring of stereocomplex crystals (SCs) with uniform dimensions (∼300 nm), which were introduced into PLLA electrospinning solution as the electrets and physical cross-linking points of high density.
View Article and Find Full Text PDFSoft Matter
January 2025
The Nonwovens Institute, NC State University, Raleigh, 27606, NC, USA.
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