Single-mode lasing of CsPbBr perovskite NWs enabled by the Vernier effect.

Nanoscale

CAS Center for Excellence in Nanoscience Beijing Key Laboratory of Micro-nano Energy and Sensor, Beijing Institute of Nanoenergy and Nanosystems Chinese Academy of Sciences, Beijing 100083, P. R. China. and School of Nanoscience and Technology, University of Chinese Academy of Sciences, Beijing 100049, P. R. China and State Key Laboratory for Mesoscopic Physics, Collaborative Innovation Centre of Quantum Matter, School of Physics, Peking University, Beijing 100871, P. R. China and Center on Nanoenergy Research, School of Physical Science and Technology, Guangxi University, Nanning, Guangxi 530004, P. R. China.

Published: March 2021

Inorganic lead halide perovskite (CsPbX3, X = Cl, Br, I) NWs (NWs) have been employed in lasers due to their intriguing attributes of tunable wavelength, low threshold, superior stability, and easy preparation. However, current CsPbX3 NW lasers usually work in a multi-mode modal, impeding their practical applications in optical communication due to the associated false signaling. In this work, high-performance single-mode lasing has been demonstrated by designing and fabricating coupled cavities in the high-quality single-crystal CsPbBr3 NWs via the focused ion beam (FIB) milling approach. The single-mode laser shows a threshold of 20.1 μJ cm-2 and a high quality factor of ∼2800 profiting from the Vernier effect, as demonstrated by the experiments and finite-different time-domain (FDTD) simulations. These results demonstrate the promising potentials of the CsPbX3 NW lasers in optical communication and integrated optoelectronic devices.

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Source
http://dx.doi.org/10.1039/d0nr08644dDOI Listing

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