Plasmon sensors respond to local changes of their surrounding environment with a shift in their resonance wavelength. This response is usually detected by measuring light scattering spectra to determine the resonance wavelength. However, single wavelength detection has become increasingly important because it simplifies the setup, increases speed, and improves statistics. Therefore, we investigated theoretically how the sensitivity toward such single wavelength scattering intensity changes depend on the material and shape of the plasmonic sensor. Surprisingly, simple equations describe this intensity sensitivity very accurately and allow us to distinguish the various contributions: Rayleigh scattering, dielectric contrast, plasmon shift, and frequency-dependent plasmon bulk damping. We find very good agreement of theoretical predictions and experimental data obtained by single particle spectroscopy.
Download full-text PDF |
Source |
---|---|
http://dx.doi.org/10.1021/acs.nanolett.0c04702 | DOI Listing |
J Hazard Mater
March 2025
Centre of Polymer and Carbon Materials, Polish Academy of Sciences, Zabrze, Poland.
In this work, the long-term degradation of polymer pellets (also known as the primary microplastics/MPs) was monitored under laboratory-controlled conditions. Polymers of different origin such as the ABS, HDPE and PA (non-processed, recycled) were exposed to demineralized and artificial seawater, stored in room (20-24 °C) and cold (4-8 °C) temperatures during 20 months period. Surface topography and thermal characteristics of selected primary MPs were examined with the use of digital microscope and thermogravimetric (TGA) analysis.
View Article and Find Full Text PDFJ Phys Condens Matter
March 2025
Department of Physics and Astronomy, University of Rochester, University of Rochester, Rochester, New York, 14627, UNITED STATES.
When compressed, certain lattices undergo phase transitions that may allow nuclei to gain sig- nificant kinetic energy. To explore the dynamics of this phenomenon, we develop a methodology to study Coulomb coupled N-body systems constrained to a sphere, as in the Thomson problem. We initialize N total Boron nuclei as point particles on the surface of the sphere, allowing them to equilibrate via Coulomb scattering with a viscous damping term.
View Article and Find Full Text PDFPhys Rev Lett
February 2025
University of Texas at Austin, Department of Physics, Austin, Texas 78712, USA.
The lowest Landau level of bilayer graphene has an octet of internal degrees of freedom, composed from spin, valley, and orbital two-level systems. Dominance of n=0 orbitals over n=1 orbitals in low energy quantum fluctuations leads to distinct fractional quantum Hall characteristics compared dominance of n=1 over n=0. The competition between n=0 and n=1 orbitals depends sensitively on particle-hole asymmetry in the single-particle Hamiltonian and on Lamb shifts due to exchange interactions with the negative energy sea, which must be accounted for simultaneously in assessing the orbital competition.
View Article and Find Full Text PDFPhys Rev Lett
February 2025
Sorbonne Université, Laboratoire Kastler Brossel, ENS-Université PSL, CNRS, Collège de France, 24 rue Lhomond, 75005, Paris, France.
We report on the imaging of the in situ spatial distribution of deterministically prepared single-atom wave packets as they expand in a plane, finding excellent agreement with the scaling dynamics predicted by the Schrödinger equation. Our measurement provides a direct and quantitative observation of the textbook free expansion of a one-particle Gaussian wave packet, which we believe has no equivalent in the existing literature. Second, we utilize these expanding wave packets as a benchmark to develop a protocol for the controlled projection of a spatially extended wave function from continuous space onto the sites of a deep optical lattice and subsequent single-atom imaging using quantum gas microscopy techniques.
View Article and Find Full Text PDFPhys Rev Lett
February 2025
S. N. Bose National Center for Basic Sciences, Department of Astrophysics and High Energy Physics, Block JD, Sector III, Salt Lake, Kolkata 700106, India.
A fundamental limitation of quantum communication is that a single qubit can carry at most one bit of classical information. For an important class of quantum communication channels, known as entanglement breaking, this limitation holds even if the sender and receiver share entangled particles. But does this mean that, for the purpose of communicating classical messages, a noisy entanglement-breaking qubit channel can be replaced by a noisy bit channel? Here we answer the question in the negative.
View Article and Find Full Text PDFEnter search terms and have AI summaries delivered each week - change queries or unsubscribe any time!