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Spatio-temporal analysis of extreme air pollution and risk assessment.
J Environ Manage
December 2024
Department of Civil Engineering, Indian Institute of Technology Indore, Simrol, Indore, 453552, Madhya Pradesh, India. Electronic address:
Extreme air pollution poses global health and environmental threats, necessitating robust policy interventions. This study first analyses the surface mass concentration of major aerosols (such as black carbon, organic carbon, dust, sea salts, and sulphates) to estimate global PM concentrations from 1980 to 2023. The developed model-estimated PM database was validated against data from 526 cities worldwide, showing strong accuracy, with RMSE, r, and R values of 7.
View Article and Find Full Text PDFArchitecting Ultra-Robust Zr(IV) Metal-Organic Framework for Energy-Efficient Desiccant Air Conditioning.
J Am Chem Soc
December 2024
School of Chemistry and Chemical Engineering, Shanghai Jiao Tong University, Shanghai 200240, China.
Air-conditioning systems, composed mainly of humidity control and heat reallocation units, play a pivotal role in upholding superior air quality and human well-being across diverse environments ranging from international space stations and pharmacies to granaries and cultural relic preservation sites, and to commercial and residential buildings. The adoption of sorbent water as the working pair and low-grade renewable or waste heat in adsorption-driven air-conditioning presents a state-of-the-art solution, notably for its energy efficiency and eco-friendliness vis-à-vis conventional electricity-driven vapor compression cycles. Here, we introduce a rational π-extension strategy to engineer an ultrarobust and highly porous zirconium metal-organic framework (Zr-MOF).
View Article and Find Full Text PDFComprehensive industry-relevant black soldier fly bioconversion characterisation by a novel chamber system.
Waste Manag
December 2024
ETH Zurich, Laboratory of Sustainable Food Processing, Schmelzbergstrasse 9 8092, Zurich, Switzerland; Singapore-ETH Centre,1 Create Way 138602, Singapore.
Black soldier fly larvae (BSFL) efficiently convert biowaste into valuable animal feed. Sustainable and reliable bioconversion is desirable to achieve optimal economic and environmental outcomes. Thus, science and industry require an accessible research platform to study complex bioconversion processes under conditions mirroring industrial-scale settings.
View Article and Find Full Text PDFDesigned Synthesis of Mesoporous sp Carbon-Conjugated Benzothiadiazole Covalent Organic Frameworks for Artificial Photosynthesis of Hydrogen Peroxide.
ACS Appl Mater Interfaces
December 2024
Hubei Key Lab on Organic and Polymeric Optoelectronic Materials, College of Chemistry and Molecular Sciences, Wuhan University, Wuhan 430072, China.
Artificial photosynthesis of hydrogen peroxide (HO) from ambient air, water, and sunlight has attracted considerable attention recently. Despite being extremely challenging to synthesis, sp carbon-conjugated covalent organic frameworks (COFs) can be powerful and efficient materials for the photosynthesis of HO due to desirable properties. Herein, we report the designed synthesis of an sp carbon-conjugated COF, BTD-spc-COF, from benzothiadiazole and triazine units with high crystallinity and ultralarge mesopores (∼4 nm).
View Article and Find Full Text PDFAssociation of social vulnerability and depression incidence post intracerebral haemorrhage: a cohort study.
BMJ Neurol Open
December 2024
Department of Neurology, Henry and Allison McCance Center for Brain Health, Mass General Brigham Inc, Boston, Massachusetts, USA.
Objectives: Survivors of intracerebral haemorrhage (ICH) are at high risk of incident depression, which is modified by social determinants of health (SDOH) and associated with worse functional outcomes. We sought to determine the role of prestroke SDOH in depression incidence after ICH to better characterise post-ICH outcomes.
Study Design: We analysed data from a cohort study of ICH survivors without prestroke depression, presenting at Massachusetts General Hospital between 2006 and 2017.
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