Few-layer and 1T-rich MoS is synthesized by a one-step solvothermal process using a rigid segment-containing polysulfide as a concomitant sulfur source and in situ intercalator. The prepared MoS displays superior hydrogen evolution reaction activity, providing a facile and mild approach for the development of high performing MoS and other two-dimensional lamellar materials.
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Polysulfide induced synthesis of a MoS self-supporting electrode with wide-layer-spacing for efficient electrocatalytic water splitting.
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Key Laboratory for Green Chemical Process of Ministry of Education, Hubei Key Laboratory for Novel Reactor and Green Chemistry Technology, Hubei Engineering Research Center for Advanced Fine Chemicals, School of Chemical Engineering and Pharmacy, Wuhan Institute of Technology, Wuhan 430073, China.
Efficient non-noble metal bifunctional electrocatalysts can increase the conversion rate of electric energy in the hydrogen evolution reaction (HER) and the oxygen evolution reaction (OER). Herein, a ball & sheet MoS/NiS composite with wide-layer-spacing and high 1T-rich MoS is assembled on nickel foam (NF) a two-step solvothermal method with polymeric sulfur (S-r-DIB) as the sulfur source. The obtained material serves as both the cathode and the anode toward overall water splitting in an alkaline electrolyte.
View Article and Find Full Text PDFConcomitant induction to few-layer and 1T-rich two-dimensional MoS by rigid segment-containing polysulfide as a sulfur source and in situ intercalator.
Chem Commun (Camb)
March 2021
Key Laboratory for Green Chemical Process of Ministry of Education, Hubei Key Laboratory for Novel Reactor and Green Chemistry Technology and School of Chemical Engineering and Pharmacy, Wuhan Institute of Technology, Wuhan 430205, P. R. China.
Few-layer and 1T-rich MoS is synthesized by a one-step solvothermal process using a rigid segment-containing polysulfide as a concomitant sulfur source and in situ intercalator. The prepared MoS displays superior hydrogen evolution reaction activity, providing a facile and mild approach for the development of high performing MoS and other two-dimensional lamellar materials.
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