We numerically study interaction of a very intense (I∼10^{17} to 5×10^{19}W/cm^{2}) femtosecond obliquely incident p-polarized laser pulse with a steep-gradient (L∼λ) plasma, i.e., within the conditions typical for modern experiments. It is shown that the hybrid stimulated Raman scattering-two-plasmon decay instability develops near the quarter-critical density surface and plays the dominant role for the plasma waves' excitation and energy absorption. The plasmons are excited as two wave packets confined near this surface with very wide ≈ω_{0}/c spatial spectra along its normal. Hence, phase-matching conditions for the 3/2 harmonic generation are fulfilled immediately and include the mechanism coming from the high harmonics of plasma waves. This mechanism has been proved experimentally by observing an additional 3/2 harmonic beam.
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http://dx.doi.org/10.1103/PhysRevE.102.063206 | DOI Listing |
Hepatol Commun
January 2025
Department of Pediatrics, Division of Gastroenterology, Hepatology, and Nutrition, Cincinnati Children's Hospital Medical Center, Cincinnati, Ohio, USA.
Acc Chem Res
December 2024
College of Chemistry, Sichuan University, Chengdu 610065, P. R. China.
Adv Sci (Weinh)
November 2024
State Key Laboratory of Structure Chemistry, Fujian Institute of Research on the Structure of Matter, Chinese Academy of Sciences, Fuzhou, Fujian, 350002, P. R. China.
To modulate nonlinear optical (NLO) effects of crystalline material holds great application potential in the photoelectronic and optical fields. Organic configurationally-locked polyene represents an exciting NLO family with large second harmonic generation (SHG) effects, whereas it is a huge blank to switch and modulate their NLO property through external stimuli. For the first time, here present unusual thermo-enhanced SHG activities are presented in a polyene-based NLO compound, 2-{3-[2-(4-pyrrolidinphenyl)vinyl]-5,5-dimethylcyclohex-2-enylidene}malononitrile (1), giving a record-high magnitude of SHG enhancement up to ≈170% during its isomorphic phase transition.
View Article and Find Full Text PDFInorg Chem
December 2024
College of Chemistry and Chemical Engineering, Qingdao University, Shandong 266071, China.
In virtue of the cationic tri(pyridin-4-yl)amine (TPA) derivatives acting as the templates, two iodometallates, [MeHTPA][CuI][CuI] () and [MeTPA][AgI] (), were constructed with different architectures. Compound features a discrete [CuI] cluster, which is further combined with [CuI] and two [MeHTPA] moieties through electrostatic interactions to result in a 3D supramolecular framework. Two types of infinite Ag-I chains with different orientations are formed in iodoargentate , and adjacent chains, together with in situ -methylated cations, are further aggregated into a final 3D supramolecule.
View Article and Find Full Text PDFAnimals (Basel)
October 2024
Department of Veterinary Clinical Sciences, School of Veterinary Medicine, Louisiana State University, Skip Bertman Drive, Baton Rouge, LA 70803, USA.
Anthropogenic activities have negatively affected many birds, including owls. The Wildlife Hospital of Louisiana (WHL) has seen a 3.2-fold increase in barred owl () cases over the past eight years (2023, 134; 2015, 42).
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