When a quantum system is subject to a thermal gradient it may sustain a steady nonequilibrium heat current by entering into a so-called nonequilibrium steady state (NESS). Here we show that NESS constitute a thermodynamic resource that can be exploited to charge a quantum battery. This adds to the list of recently reported sources available at the nanoscale, such as coherence, entanglement, and quantum measurements. We elucidate this concept by showing analytic and numerical studies of a two-qubit quantum battery that is alternatively charged by an incoherent heat flow and discharged by application of a properly chosen unitary gate. The presence of a NESS for the charging step guarantees steady operation with positive power output. Decreasing the duration of the charging step results in a time-periodic steady state accompanied by increased efficiency and output power. The device is amenable to implementation with different nanotechnology platforms.
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http://dx.doi.org/10.1103/PhysRevE.102.062133 | DOI Listing |
Macromol Rapid Commun
January 2025
Institut für Chemie, Technische Universität Chemnitz, Straße der Nationen 62, 09111, Chemnitz, Germany.
Aromatic diimides such as naphthalene diimide (NDI) and pyromellitic diimide (MDI) are important building blocks for organic electrode materials. They feature a two-electron redox mechanism that allows for energy storage. Due to the smaller size of MDI compared to NDI its theoretical capacity is higher.
View Article and Find Full Text PDFSmall
January 2025
Key Laboratory of Advanced Technologies of Materials, Ministry of Education, School of Materials Science and Engineering, Southwest Jiaotong University, Chengdu, 610031, China.
A novel polymer electrolyte based on CsPbI quantum dots (QDs) reinforced polyacrylonitrile (PAN), named as PIL, is exploited to address the low room-temperature (RT) ion conductivity and poor interfacial compatibility of polymer solid-state electrolytes. After optimizing the content of CsPbI QDs, RT ion conductivity of PIL largely increased from 0.077 to 0.
View Article and Find Full Text PDFNanomaterials (Basel)
December 2024
Quantum Nano Centre, Department of Chemical Engineering, University of Waterloo, Waterloo, ON N2L 3G1, Canada.
Laser conversion of commercial polymers to laser-induced graphene (LIG) using inexpensive and accessible CO lasers has enabled the rapid prototyping of promising electronic and electrochemical devices. Frequently used to pattern interdigitated supercapacitors, few approaches have been developed to pattern batteries-in particular, full cells. Herein, we report an LIG-based approach to a planar, interdigitated Li-S battery.
View Article and Find Full Text PDFSmall
January 2025
Fujian Provincial Key Laboratory of Quantum Manipulation and New Energy Materials, College of Physics and Energy, Fujian Normal University, Fuzhou, Fujian, 350117, China.
Single-atom materials provide a platform to precisely regulate the electrochemical redox behavior of electrode materials with atomic level. Here, a multifield-regulated sintering route is reported to rapidly prepare single-atom zinc with a very high loading mass of 24.7 wt.
View Article and Find Full Text PDFNat Commun
January 2025
State Key Laboratory of Millimeter Waves, School of Information Science and Engineering, Southeast University, Nanjing, China.
Microwave-optical interaction and its effective utilization are vital technologies at the frontier of classical and quantum sciences for communication, sensing, and imaging. Typically, state-of-the-art microwave-to-optical converters are realized by fiber and circuit approaches with multiple processing steps, and external powers are necessary, which leads to many limitations. Here, we propose a programmable metasurface that can achieve direct and high-speed free-space microwave-to-laser conversion.
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