The spin of a single electron in a semiconductor quantum dot provides a well-controlled and long-lived qubit implementation. The electron charge in turn allows control of the position of individual electrons in a quantum dot array, and enables charge sensors to probe the charge configuration. Here we show that the Coulomb repulsion allows an initial charge transition to induce subsequent charge transitions, inducing a cascade of electron hops, like toppling dominoes. A cascade can transmit information along a quantum dot array over a distance that extends by far the effect of the direct Coulomb repulsion. We demonstrate that a cascade of electrons can be combined with Pauli spin blockade to read out distant spins and show results with potential for high fidelity using a remote charge sensor in a quadruple quantum dot device. We implement and analyse several operating modes for cascades and analyse their scaling behaviour. We also discuss the application of cascade-based spin readout to densely-packed two-dimensional quantum dot arrays with charge sensors placed at the periphery. The high connectivity of such arrays greatly improves the capabilities of quantum dot systems for quantum computation and simulation.
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http://dx.doi.org/10.1038/s41467-020-20388-6 | DOI Listing |
R Soc Open Sci
January 2025
Pharmaceutical Analytical Chemistry Department, Faculty of Pharmacy, Cairo University, Cairo 11562, Egypt.
Carbon quantum dots (CQDs) are a recently developed class of fluorescent nanoparticles made from carbon. Co-doping with heteroatoms such as nitrogen and sulfur improved the properties and generated a high quantum yield. In the proposed study, we utilized a simple, cost-effective, single-stage hydrothermal approach to produce extreme photoluminescence co-doped, nitrogen and sulfur, CQDs (N,S-CODs).
View Article and Find Full Text PDFTurk J Chem
November 2024
School of Chemical and Blasting Engineering, Anhui University of Science and Technology, Huainan, P.R. China.
The development of ultraviolet (UV) shielding materials is of great importance to protect human health and prevent the degradation of organic matter. However, the synthesis of highly efficient UV shielding polymer nanocomposites is currently limited by the agglomeration of inorganic anti-UV nanoparticles (NPs) within the polymer matrix and the limited absorption spectrum of UV shielding agents. In this study, highly effective manganese doped carbon quantum dots@halloysite nanotube composites (Mn-CDs@HNTs/PAS) were successfully synthesized by loading manganese-doped carbon quantum dots (Mn-CDs) into UV shielding effective halloysite nanotubes (HNTs) via the solvothermal method, followed by polymerization modification (PAS).
View Article and Find Full Text PDFSmall
January 2025
Chair for Emerging Electronic Technologies, TUD Dresden University of Technology, Nöthnitzer Straße 61, 01187, Dresden, Germany.
The stability of perovskite quantum dot solar cells is one of the key challenges of this technology. This study reveals the unique degradation behavior of cesium lead triiodide (CsPbI) quantum dot solar cells. For the first time, it is shown that the oxygen-induced degradation and performance loss of CsPbI quantum dot photovoltaic devices can be reversed by exposing the degraded samples to humidity, allowing the performance to recover and even surpass the initial performance.
View Article and Find Full Text PDFJ Phys Chem Lett
January 2025
Department of Chemistry, Yonsei University, Wonju, Gangwon 26493, Korea.
Understanding the environment-dependent stability and photoluminescence (PL) properties of advanced perovskite materials remains a challenge with conflicting views. Herein, we investigated the influence of the host matrix (poly(methyl methacrylate) (PMMA) and polystyrene (PS)) and atmospheric conditions (ambient and N) on the PL properties of a CsPbBr perovskite quantum dot (PQD) using single-particle spectroscopy. Despite the same PL blinking mechanism, the PL properties of the PQD were considerably affected by the environmental conditions.
View Article and Find Full Text PDFSmall
January 2025
Department of Physics, Malaviya National Institute of Technology Jaipur, Rajasthan, 302017, India.
Increasing attention to sustainability and cost-effectiveness in energy storage sector has catalyzed the rise of rechargeable Zinc-ion batteries (ZIBs). However, finding replacement for limited cycle-life Zn-anode is a major challenge. Molybdenum disulfide (MoS), an insertion-type 2D layered material, has shown promising characteristics as a ZIB anode.
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