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Synthesis of TEMPO radical decorated hollow porous aromatic frameworks for selective oxidation of alcohols. | LitMetric
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Synthesis of TEMPO radical decorated hollow porous aromatic frameworks for selective oxidation of alcohols.

Yan-Ming Shen Yun Xue Mi Yan Hui-Ling Mao Hu Cheng Zhuo Chen Zhi-Wei Sui Shao-Bin Zhu Xiu-Jun Yu Jin-Liang Zhuang

Chem Commun (Camb)

School of Chemistry and Materials Science, Key Lab for Functional Materials Chemistry of Guizhou Province, Guizhou Normal University, 116 Baoshan Road North, Guiyang 550001, P. R. China and NanoFCM INC., Xiamen Pioneering Park for Overseas Chinese Scholars, Xiamen, 361005, P. R. China.

Published: January 2021

AI Article Synopsis

  • A bottom-up method was created to produce hollow aromatic frameworks (HPAF-TEMPO) using functionalized monomers and SiO2 nanospheres as templates.
  • These frameworks have a high concentration of TEMPO sites and unique pore structures that enhance their effectiveness.
  • The HPAF-TEMPO framework efficiently oxidizes a variety of alcohols, achieving great selectivity in the process.

Article Abstract

A bottom-up approach was developed to prepare TEMPO radical decorated hollow aromatic frameworks (HPAF-TEMPO) by using TEMPO radical functionalized monomers and SiO2 nanospheres as templates. The accessible inner layer, high density of TEMPO sites, and hybrid micro-/mesopores of the HPAF-TEMPO enable the aerobic oxidation of a broad range of alcohols with high efficiency and excellent selectivity.

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 Source
http://dx.doi.org/10.1039/d0cc06965eDOI Listing

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