The ubiquity of wearables, coupled with the increasing demand for power, presents a unique opportunity for nanostructured fiber-based mobile energy storage systems. When designing wearable electronic textiles, there is a need for mechanically flexible, low-cost and light-weight components. To meet this demand, we have developed an all-in-one fiber supercapacitor with a total thickness of less than 100 μm using a novel facile coaxial wet-spinning approach followed by a fiber wrapping step. The formed triaxial fiber nanostructure consisted of an inner poly(3,4-ethylenedioxythiophene) polystyrene sulfonate (PEDOT:PSS) core coated with an ionically conducting chitosan sheath, subsequently wrapped with a carbon nanotube (CNT) fiber. The resulting supercapacitor is highly flexible, delivers a maximum energy density 5.83 Wh kg and an extremely high power of 1399 W kg along with remarkable cyclic stability and specific capacitance. This asymmetric all-in-one fiber supercapacitor may pave the way to a future generation of wearable energy storage devices.
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http://dx.doi.org/10.3390/nano11010003 | DOI Listing |
ACS Nano
January 2025
Nano Hybrid Technology Research Center, Korea Electrotechnology Research Institute (KERI), Changwon 51543, Republic of Korea.
Hydrogen-bond-driven 1D assembly of carbon nanotubes dispersed in organic solvents remains challenging owing to difficulties associated with achieving high oxidation levels and uniform dispersion. Here, we introduced a bioinspired wet-spinning method that utilizes highly oxidized single-walled carbon nanotubes dispersed in organic solvents without superacid or dispersants. By incorporating submicrometer-sized graphene oxide nanosheets, we facilitated the ejection of 1.
View Article and Find Full Text PDFSmall
January 2025
National Engineering Lab for Textile Fiber Materials & Processing Technology, Zhejiang Sci-Tech University, Hangzhou, 310018, P. R. China.
2D materials feature large specific surface areas and abundant active sites, showing great potential in energy storage and conversion. However, the dense, stacked structure severely restricts its practical application. Inspired by the structure of bamboo in nature, hollow interior and porous exterior wall, hollow MXene aerogel fiber (HA-TiCT fiber) is proposed.
View Article and Find Full Text PDFNanomaterials (Basel)
December 2024
Department of Energy and Power Engineering, North University of China, Taiyuan 038507, China.
The NiCoO Nanosheets@Carbon fibers composites have been successfully synthesized by a facile co-electrodeposition process. The mesoporous NiCoO nanosheets aligned vertically on the surface of carbon fibers and crosslinked with each other, producing loosely porous nanostructures. These hybrid composite electrodes exhibit high specific capacitance in a three-electrode cell.
View Article and Find Full Text PDFMaterials (Basel)
December 2024
Shandong Jinhong New Material Co. Ltd., Weifang 262100, China.
Nitrogen-doped graphene quantum dots (N-GQDs) are widely used in biosensing, catalysis, and energy storage due to their excellent conductivity, high specific surface area, unique quantum size effects, and optical properties. In this paper, we successfully synthesized N-GQDs using a facile hydrothermal approach and investigated the effects of different hydrothermal temperatures and times on the morphology and structure of N-GQDs. The results indicated that the size of N-GQDs gradually increased and they eventually aggregated into graphene fragments with increasing temperature or reaction time.
View Article and Find Full Text PDFSmall
January 2025
State Key Laboratory of Silicon and Advanced Semiconductor Materials, School of Materials Science and Engineering, Zhejiang University, Hangzhou, 310058, China.
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