The adverse effects of air pollution on respiratory health make air quality monitoring with high spatial and temporal resolutions essential especially in cities. Despite considerable interest and efforts, the application of various types of sensors is considered immature owing to insufficient sensitivity and cross-interference under ambient conditions. Here, a fully integrated chemiresistive sensor array (CSA) with parts-per-trillion sensitivity is demonstrated with its application for on-road NO monitoring. An analytical model is suggested to describe the kinetics of the sensor responses and quantify molecular binding affinities. Finally, the full characterization of the system is connected to implement on-road measurements on NO vapor with quantification as its ultimate field application. The obtained results suggest that the CSA shows potential as an essential unit to realize an air-quality monitoring network with high spatial and temporal resolutions.
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http://dx.doi.org/10.1002/advs.202002014 | DOI Listing |
Sensors (Basel)
January 2025
Institute of Physics, University of Tartu, EE-50411 Tartu, Estonia.
Low-power gas sensors that can be used in IoT (Internet of Things) systems, consumer devices, and point-of-care devices will enable new applications in environmental monitoring and health protection. We fabricated a monolithic chemiresistive gas sensor by integrating a micro-lightplate with a 2D sensing material composed of single-layer graphene and monolayer-thick TiO. Applying ultraviolet (380 nm) light with quantum energy above the TiO bandgap effectively enhanced the sensor responses.
View Article and Find Full Text PDFAdv Sci (Weinh)
January 2025
Data61, CSIRO, Clayton, VIC, 3168, Australia.
The rapid growth of Internet of Things (IoT) devices necessitates efficient data compression techniques to manage the vast amounts of data they generate. Chemiresistive sensor arrays (CSAs), a simple yet essential component in IoT systems, produce large datasets due to their simultaneous multi-sensor operations. Classical principal component analysis (cPCA), a widely used solution for dimensionality reduction, often struggles to preserve critical information in complex datasets.
View Article and Find Full Text PDFNanomicro Lett
January 2025
College of Mechanical Engineering, Yangzhou University, Yangzhou, 225127, People's Republic of China.
The integration of dual-mesoporous structures, the construction of heterojunctions, and the incorporation of highly concentrated oxygen vacancies are pivotal for advancing metal oxide-based gas sensors. Nonetheless, achieving an optimal design that simultaneously combines mesoporous structures, precise heterojunction modulation, and controlled oxygen vacancies through a one-step process remains challenging. This study proposes an innovative method for fabricating zinc stannate semiconductors featuring dual-mesoporous structures and tunable oxygen vacancies via a direct solution precursor plasma spray technique.
View Article and Find Full Text PDFDalton Trans
January 2025
Department of Chemistry, Central Tribal University of Andhra Pradesh (CTUAP), Andhra Pradesh, 535003, India.
Hydrogen is a zero-emissive fuel and has immense potential to replace carbon-emitting fuels in the future. The development of efficient H sensors is essential for preventing hazardous situations and facilitating the widespread usage of hydrogen. Chemiresistors are popular gas sensors owing to their attractive properties such as fast response, miniaturization, simple integration with electronics and low cost.
View Article and Find Full Text PDFJ Hazard Mater
January 2025
School of Integrated Circuits, Dalian University of Technology, Dalian, Liaoning 116024, China. Electronic address:
Tellurium nanotubes (TeNT) heterojunction with Tellurium oxide (TeO) were prepared by in situ oxidation at elevated temperatures in air. The chemiresistive type NO sensor was then fabricated by depositing the synthesized TeNT/TeO on the integrated gold electrodes. The response of the TeNT/TeO based sensor to 600 ppb NO was 38.
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