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Graphene oxide transport and retention in biochar media. | LitMetric

Graphene oxide transport and retention in biochar media.

Chemosphere

Department of Civil and Environmental Engineering, South Dakota School of Mines and Technology, 501 East Saint Joseph Street, Rapid City, SD, 57701, United States; 2-Dimensional Materials for Biofilm Engineering Science and Technology (2DBEST) Center, South Dakota School of Mines and Technology, 501 East Saint Joseph Street, Rapid City, SD, 57701, United States.

Published: February 2021

AI Article Synopsis

Article Abstract

This study explores the use of biochar (BC), an inexpensive filtration media, for removing graphene oxide (GO) contaminants from the aquatic subsurface environments. Mass balance approaches and column dissection tests were used to analyze the retention behavior of GO in a series of model fixed-bed columns as a function of ionic strength (IS) and flowrate. The column based on the biochar media (BC) displayed 3.6-fold higher retention compared to the quartz sand (control). To overcome the challenges of unfavorable electrostatic interactions between GO and BC, we used a facile functionalization strategy to modify the BC surfaces with nanoscale zero-valent iron (BC-nZVI). The BC-nZVI (5:1, w/w) retained 2.6-fold higher amounts of GO compared with bare biochar. Furthermore, the performance of BC-nZVI increased with decreasing values of IS, attributed to the attachment of GO to nZVI where nZVI was partially dissolved by the presence of higher chloride ion at high IS. A better GO retention (86%) at higher IS was observed in BC where the GO was primarily retained due to the higher aggregation via straining.

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Source
http://dx.doi.org/10.1016/j.chemosphere.2020.128397DOI Listing

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