Quantum state tomography (QST) has been the traditional method for characterization of an unknown state. Recently, many direct measurement methods have been implemented to reconstruct the state in a resource efficient way. In this Letter, we present an interferometric method, in which any qubit state, whether mixed or pure, can be inferred from the visibility, phase shift, and average intensity of an interference pattern using a single-shot measurement-hence, we call it quantum state interferography. This provides us with a "black box" approach to quantum state estimation, wherein, between the incidence of the photon and extraction of state information, we are not changing any conditions within the setup, thus giving us a true single shot estimation of the quantum state. In contrast, standard QST requires at least two measurements for pure state qubit and at least three measurements for mixed state qubit reconstruction. We then go on to show that QSI is more resource efficient than QST for quantification of entanglement in pure bipartite qubits. We experimentally implement our method with high fidelity using the polarization degree of freedom of light. An extension of the scheme to pure states involving d-1 interferograms for d-dimensional systems is also presented. Thus, the scaling gain is even more dramatic in the qudit scenario for our method, where, in contrast, standard QST, without any assumptions, scales roughly as d^{2}.
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http://dx.doi.org/10.1103/PhysRevLett.125.123601 | DOI Listing |
Nat Commun
January 2025
School of Environment, Tsinghua University, Beijing, 100084, P. R. China.
Modulation of electronic spin states in cobalt-based catalysts is an effective strategy for molecule activations. Crystalline-amorphous interfaces often exhibit unique catalytic properties due to disruptions of long-range order and alterations in electronic structure. However, the mechanisms of molecule activation and spin states at interfaces remain elusive.
View Article and Find Full Text PDFJ Colloid Interface Sci
January 2025
State Key Laboratory of Bio-Fibers and Eco-Textiles, Qingdao University, No. 308 Ningxia Road, Qingdao 266071 PR China. Electronic address:
Luminescent solar concentrators (LSCs) are large scale sunlight collector and can be used for building-integrated photovoltaics (BIPV). Achieving high-performance LSCs requires fluorophores with broad absorption, high quantum yield and a large Stokes shift. Nevertheless, conventional high-efficiency LSCs typically rely on heavy metal-based quantum dots as fluorophores.
View Article and Find Full Text PDFBiosens Bioelectron
January 2025
Catalan Institute of Nanoscience and Nanotechnology (ICN2), CSIC and BIST, Campus UAB, Bellaterra, Barcelona, 08193, Spain; Catalan Institution for Research and Advanced Studies (ICREA) Passeig de Lluís Companys, 23, Barcelona, 08010, Spain. Electronic address:
Quantum dots (QDs) are the smallest nanomaterials (2-10 nm), with unique optical and electronic properties. Thanks to these properties, QDs have been standing during the last years as signal tags for different applications, including bioimaging, fluorescent biosensors and electrochemical assays. In this review, we explore the current state-of-the art on these nanomaterials, differentiating them between semiconductor and carbon-based QDs.
View Article and Find Full Text PDFJ Phys Chem A
January 2025
Department of Chemistry and Supercomputing Institute, University of Minnesota, Minneapolis, Minnesota 55455-0431, United States.
The energy gaps, spin-orbit coupling (SOC), and admixture coefficients over a series of the configurations are evaluated by the SA-CASSCF/6-31G, SA-CASSCF/6-31G*, SA-CASSCF/ANO-RCC-VDZP, and MS-CASPT2/ANO-RCC-VDZP to reveal the extent of the inaccuracy of the SA-CASSCF. By comparing the mean absolute errors for the energy gaps and the admixture coefficient magnitudes (ACMs) measured between the SA-CASSCF/6-31G, SA-CASSCF/6-31G*, or SA-CASSCF/ANO-RCC-VDZP and the MS-CASPT2/ANO-RCC-VDZP, the SA-CASSCF/6-31G is selected as the electronic structure method in the nonadiabatic molecular dynamics simulation. The major components of the ACMs of the SA-CASSCF/6-31G and MS-CASPT2/ANO-RCC-VDZP are identified and compared; we find that the ACMs are underestimated by the SA-CASSCF/6-31G, which is verified by the reasonable triplet quantum yield simulated by the trajectory surface hopping and the calibrated SA-CASSCF/6-31G.
View Article and Find Full Text PDFSci Rep
January 2025
Laboratory of Pharmacology, Department of Pharmacy, Faculty of Pharmaceutical Sciences, Tokyo University of Science, Chiba, Japan.
Recently, exposure to sounds with ultrasound (US) components has been shown to modulate brain activity. However, the effects of US on emotional states remain poorly understood. We previously demonstrated that the olfactory bulbectomized (OBX) rat depression model is suitable for examining the effects of audible sounds on emotionality.
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