This study investigated whether bioaugmentation improves sulfamethoxazole (SMX) degradation and nitrogen removal in the Moving Bed Biofilm Reactor (MBBR) system. The effects of the C/N ratio on SMX degradation and nitrogen removal were also evaluated. Using MBBR system operation experiments, the bioaugmented reactor was found to perform more effectively than the non-bioaugmentation reactor, with the highest SMX, nitrate-N, and ammonia-N removal efficiencies of 80.49, 94.70, and 96.09%, respectively. The changes in the sulfonamide resistance genes and bacterial communities were detected at various operating conditions. The results indicate that the diversity of the bacterial communities and the abundance of resistance genes were markedly influenced by bioaugmentation and the C/N ratio, with Achromobacter among the dominant genera in the MBBR system. The bio-toxicity of samples, calculated as the inhibition percentage (IP) toward Escherichia coli, was found to decrease to non-toxic ranges after treatment.
Download full-text PDF |
Source |
---|---|
http://dx.doi.org/10.1016/j.ecoenv.2020.111258 | DOI Listing |
J Colloid Interface Sci
December 2024
Guangdong Key Laboratory of Environmental Catalysis and Health Risk Control, School of Environmental Science and Engineering, Institute of Environmental Health and Pollution Control, Guangdong University of Technology, Guangzhou 510006, China.
Developing advanced heterogeneous catalysts through structural modifications effectively enhances the catalytic activity of non-homogeneous catalysts for removing emerging micropollutants (EMPs). In this study, MoTiCT@Co with Mo vacancies was synthesized using the Lewis molten salt method, which efficiently activates peroxymonosulfate (PMS) and continuously degrades EMPs in water. The abundant Mo vacancy structure in the material acts as an anchoring site for Co nanoparticles and a co-catalytic site for Fenton-like reactions, enabling PMS adsorption and activation.
View Article and Find Full Text PDFCarbohydr Polym
March 2025
School of Environmental and Architecture, University of Shanghai for Science and Technology, Shanghai 200093, China. Electronic address:
Carbon dots (CDs) mediated g-CN (CN) is a promising visible-light-driven semiconductor in catalyzing peroxymonosulfate (PMS) for aqueous contaminants remediation. However, the poor dispersibility of powered catalyst and its challenging recyclability impede their broader application. Herein, we embedded FeN bridge within the g-CN framework and immobilized g-CN gel beads (CA/FNCCN) through a 3D cross-linking process with sodium alginate.
View Article and Find Full Text PDFInt J Mol Sci
December 2024
School of Agricultural Engineering and Food Science, Shandong University of Technology, Zibo 255000, China.
In the electrocatalytic (EC) degradation process, challenges such as inefficient mass transfer, suboptimal mineralization rates, and limited current efficiency have restricted its broader application. To overcome these obstacles, this study synthesized spherical particle electrodes (FeNi@BC) with superior electrocatalytic performance using a bio-inspired preparation method. A three-dimensional electrocatalytic oxidation system based on FeNi@BC electrode, EC/FeNi@BC, showed excellent degradation efficiency of sulfamethoxazole (SMX), reaching 0.
View Article and Find Full Text PDFEnviron Res
December 2024
School of Environment and Architecture, University of Shanghai for Science and Technology, 516 Jungong Rd., Shanghai, 200093, PR China. Electronic address:
The technology to solve the problem of the efficient pollutant removal in peroxymonosulfate (PMS) activation was the ultimate goal. There was an urgent need to achieving higher catalytic activity and oxidation efficiency. Herein, we present a MgAl-based layered double hydroxide assembled as a 2D confined catalyst (MgAl-Co-LDH) with Co metal in chelated form (Co-EDTA) for highly efficient PMS activation degrading sulfamethoxazole (SMX).
View Article and Find Full Text PDFEnviron Technol
December 2024
School of Environmental Science and Engineering, Southwest Jiaotong University, Chengdu, People's Republic of China.
Ascorbic acid (AA) was used as a reducing agent to improve the Fe(III)-activated peracetic acid (PAA) system for the removal of sulfamethoxazole (SMX) in this work. The efficiency, influencing factors and mechanism of SMX elimination in the AA/Fe(III)/PAA process were studied. The results exhibited that AA facilitated the reduction of Fe(III) to Fe(II) and subsequently improved the activation of PAA and HO.
View Article and Find Full Text PDFEnter search terms and have AI summaries delivered each week - change queries or unsubscribe any time!