Topology and strong electron correlations are crucial ingredients in emerging quantum materials, yet their intersection in experimental systems has been relatively limited to date. Strongly correlated Weyl semimetals, particularly when magnetism is incorporated, offer a unique and fertile platform to explore emergent phenomena in novel topological matter and topological spintronics. The antiferromagnetic Weyl semimetal MnSn exhibits many exotic physical properties such as a large spontaneous Hall effect and has recently attracted intense interest. In this work, we report synthesis of epitaxial Mn Sn films with greatly extended compositional range in comparison with that of bulk samples. As Sn atoms are replaced by magnetic Mn atoms, the Kondo effect, which is a celebrated example of strong correlations, emerges, develops coherence, and induces a hybridization energy gap. The magnetic doping and gap opening lead to rich extraordinary properties, as exemplified by the prominent DC Hall effects and resonance-enhanced terahertz Faraday rotation.
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http://dx.doi.org/10.1126/sciadv.abc1977 | DOI Listing |
Phys Rev Lett
November 2024
School of Physical Science and Technology, ShanghaiTech University, Shanghai 201210, China.
Generally, the dissipationless Hall effect in solids requires time-reversal symmetry breaking (TRSB), where TRSB induced by external magnetic field results in the ordinary Hall effect, while TRSB caused by spontaneous magnetization gives rise to the anomalous Hall effect (AHE) which scales with the net magnetization. The AHE is therefore not expected in antiferromagnets with vanishing small magnetization. However, large AHE was recently observed in certain antiferromagnets with noncollinear spin structure and nonvanishing Berry curvature.
View Article and Find Full Text PDFNat Nanotechnol
December 2024
The Institute for Solid State Physics, The University of Tokyo, Kashiwa, Japan.
Spintronics based on ferromagnets has enabled the development of microwave oscillators and diodes. To achieve even faster operation, antiferromagnets hold great promise despite their challenging manipulation. So far, controlling antiferromagnetic order with microwave currents remains elusive.
View Article and Find Full Text PDFJ Phys Condens Matter
November 2024
Department of Physics, Indian Institute of Technology, Kanpur 208016, India.
GdSiAl single crystal has been investigated by means of magnetic and magneto-transport measurements and compared withdensity functional theory (DFT) calculations. Significant non-saturating magnetoresistance reaching∼18%at 12T and2Kwas observed, alongside the presence of Shubnikov-de Haas oscillations with the fundamental frequencies 22.09T and 77.
View Article and Find Full Text PDFJ Phys Condens Matter
November 2024
Department of Condensed Matter and Materials Physics, S. N. Bose National Centre for Basic Sciences, Kolkata, West Bengal 700106, India.
Magnetic topological semimetals are manifestations of the interplay between electronic and magnetic phases of matter, leading to peculiar characteristics such as the anomalous Hall effect (AHE) and the topological Hall effect (THE). MnSn is a time-reversal symmetry-broken magnetic Weyl semimetal showing topological characteristics within the Kagome lattice network. This study reveals a large THE in MnSn (6% Mn deficit MnSn) at room temperature in the-plane, despite being an antiferromagnet.
View Article and Find Full Text PDFJ Phys Condens Matter
November 2024
Department of Electronic Science and Engineering, Tianjin Key Laboratory of Efficient Utilization of Solar Energy, Engineering Research Center of Thin Film Optoelectronics Technology (Ministry of Education), Nankai University, Tianjin 300350, People's Republic of China.
Realizing novel two-dimensional (2D) magnetic states would accelerate the development of advanced spintronic devices and the understandings of 2D magnetic physics. In this paper, we have examined the magnetic and electronic properties of 20 dynamically stable and exfoliable MXO (M = Ti-Ni; X = S-Te; excluding CoTeO). It has been unveiled that [XO]-and [M]-crystal fields govern the M-3orbital splittings in MXO.
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