Background: Satellite imagery will offer unparalleled global spatial coverage at high-resolution for long term cost-effective monitoring of CO concentration plumes generated by emission hotspots. CO emissions can then be estimated from the magnitude of these plumes. In this paper, we assimilate pseudo-observations in a global atmospheric inversion system to assess the performance of a constellation of one to four sun-synchronous low-Earth orbit (LEO) imagers to monitor anthropogenic CO emissions. The constellation of imagers follows the specifications from the European Spatial Agency (ESA) for the Copernicus Anthropogenic Carbon Dioxide Monitoring (CO2M) concept for a future operational mission dedicated to the monitoring of anthropogenic CO emissions. This study assesses the uncertainties in the inversion estimates of emissions ("posterior uncertainties").
Results: The posterior uncertainties of emissions for individual cities and power plants are estimated for the 3 h before satellite overpasses, and extrapolated at annual scale assuming temporal auto-correlations in the uncertainties in the emission products that are used as a prior knowledge on the emissions by the Bayesian framework of the inversion. The results indicate that (i) the number of satellites has a proportional impact on the number of 3 h time windows for which emissions are constrained to better than 20%, but it has a small impact on the posterior uncertainties in annual emissions; (ii) having one satellite with wide swath would provide full images of the XCO plumes, and is more beneficial than having two satellites with half the width of reference swath; and (iii) an increase in the precision of XCO retrievals from 0.7 ppm to 0.35 ppm has a marginal impact on the emission monitoring performance.
Conclusions: For all constellation configurations, only the cities and power plants with an annual emission higher than 0.5 MtC per year can have at least one 8:30-11:30 time window during one year when the emissions can be constrained to better than 20%. The potential of satellite imagers to constrain annual emissions not only depend on the design of the imagers, but also strongly depend on the temporal error structure in the prior uncertainties, which is needed to be objectively assessed in the bottom-up emission maps.
Download full-text PDF |
Source |
---|---|
http://www.ncbi.nlm.nih.gov/pmc/articles/PMC7650226 | PMC |
http://dx.doi.org/10.1186/s13021-020-00153-4 | DOI Listing |
J Cancer Res Clin Oncol
January 2025
Department of Medical Oncology, Cancer Center, West China Hospital, Sichuan University, 37 Guoxue Alley, Chengdu, Sichuan, 610041, China.
Purpose: To evaluate the added value of additional Ga-FAPI PET/CT following CT for primary staging, detection of postoperative recurrence, and management of gastric cancer patients.
Methods: We retrospectively included patients with gastric cancers who underwent contrast-enhanced computed tomography (ceCT), followed by Ga-FAPI PET/CT within 30 days. Ga-FAPI PET/CT was performed for initial staging or detection of postoperative recurrence.
Mikrochim Acta
January 2025
Department of Pharmacology and Therapeutics, Faculty of Veterinary Medicine, Damanhour University, Damanhour, 22511, AlBeheira, Egypt.
The hydrothermal synthesis is presented of copper-doped carbon dots (Cu-CDs) from citric acid, urea, and copper chloride, resulting in blue-fluorescent particles with stable emission at 438 nm when excited at 340 nm. Through comprehensive spectroscopic and microscopic characterization (FTIR, XPS, UV, and HRTEM), the Cu-CDs demonstrated remarkable stability across varying pH levels, ionic strengths, temperatures, and UV exposure. Notably, Cu-CDs exhibit ultra-sensitive and selective detection of hexavalent chromium [Cr(VI)] ions in aqueous environments driven by fluorescence quenching.
View Article and Find Full Text PDFAngew Chem Int Ed Engl
January 2025
Zhengzhou University, College of Chemistry and Molecular Engineering, CHINA.
Time-dependent afterglow colored (TDAC) behavior differs from static afterglow by involving wavelength changes, enabling low-cost, high-level encryption and anti-counterfeiting. However, the existing carbon dot (CD)-based TDAC materials lack a clear mechanistic explanation and controllable wavelength changes, significantly hindering the progress of practical applications in this field. In this study, we synthesized CDs composites with customizable tunable TDAC wavelengths across the visible region.
View Article and Find Full Text PDFACS Sens
January 2025
Department of Mechanical Engineering, University of British Columbia, 2054-6250 Applied Science Lane, Vancouver, British Columbia V6T 1Z4, Canada.
Natural gas (NG) is a promising alternative to diesel for sustainable transport, potentially reducing GHG and air quality emissions significantly. However, the GHG benefits hinge on managing methane slip, the unburned methane in the exhaust of NG engines, which carries a significant global warming potential. The CH slip from NG engines is highly dependent on engine type and operation, and effective greenhouse gas emission mitigation requires that the actual operation of real-world engines is monitored.
View Article and Find Full Text PDFInt J Biol Macromol
January 2025
State Key Laboratory of Biobased Fiber Manufacturing Technology, Tianjin University of Science and Technology, Tianjin 300457, PR China; Tianjin Key Laboratory of Pulp and Paper, Tianjin University of Science and Technology, Tianjin 300457, PR China; China Light Industry Key Laboratory of Papermaking and Biorefinery, Tianjin University of Science and Technology, Tianjin 300457, PR China. Electronic address:
Developing sensitive and reliable methods for detecting antibiotics in water solutions is essential for protecting public health and the environment. Here, we report a novel fluorescent film with superior mechanical properties and detection response to ciprofloxacin (CIP), achieved through the in-situ growth of europium-based metal-organic frameworks on TEMPO-oxidized cellulose nanofibrils (TOCNF). Firstly, Eu(III) and 2,6-pyridinedicarboxylic acid (DPA) served as precursors, and a simple self-assembly strategy was employed to grow the composite film material (Eu-DPA@TOCNF) in situ on TOCNF, which exhibited characteristic emission peaks.
View Article and Find Full Text PDFEnter search terms and have AI summaries delivered each week - change queries or unsubscribe any time!