The generation of few-cycle laser pulses proved to be a key enabling technology in strong-field physics and ultrafast science. The question naturally arises whether one can induce few-cycle localized plasmon oscillations in optical near-fields. Here, we perform a comparative study of different plasmonic nanoresonators illuminated by few-cycle pulses. We analyze the number of cycles (NOC) of the plasmonic field, the near-field enhancement (NFE) as well as the figure of merit NFE/NOC. The pulse length dependence of these quantities is also investigated. Throughout the inspected pulse-length interval silica-gold and silica-silver core-shell monomers have the potential to preserve the NOC of the incoming pulse, silver bow-ties result in the highest NFE, whereas gold core-shell dimers have the highest NFE/NOC. Based on the analysis, silver bow-ties, gold core-shell and silver nanorod dimers proved to be the most suitable for few-cycle near-field amplification.
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http://dx.doi.org/10.1038/s41598-020-69761-x | DOI Listing |
Nat Commun
August 2024
Max-Born-Institut für Nichtlineare Optik und Kurzzeitspektroskopie, Max-Born-Strasse 2A, 12489, Berlin, Germany.
The coupling of circularly polarized light to local band structure extrema ("valleys") in two dimensional semiconductors promises a new electronics based on the valley degree of freedom. Such pulses, however, couple only to valley charge and not to the valley current, precluding lightwave manipulation of this second vital element of valleytronic devices. Contradicting this established wisdom, we show that the few cycle limit of circularly polarized light is imbued with an emergent vectorial character that allows direct coupling to the valley current.
View Article and Find Full Text PDFAdv Mater
June 2024
Dresden Integrated Center for Applied Physics and Photonic Materials (IAPP), Technische Universität Dresden, Hermann-Krone-Bau, Nöthnitzer Str. 61, 01187, Dresden, Germany.
Organic semiconductors provide the potential of biodegradable technologies, but prototypes do only rarely exist. Transparent, ultrathin programmable luminescent tags (PLTs) are presented for minimalistic yet efficient information storage that are fully made from biodegradable or at least industrially compostable, ready-to-use materials (bioPLTs). As natural emitters, the quinoline alkaloids show sufficient room temperature phosphorescence when being embedded in polymer matrices with cinchonine exhibiting superior performance.
View Article and Find Full Text PDFNano Lett
May 2024
Max Planck Institute of Quantum Optics, Hans-Kopfermann-Str. 1, 85478 Garching, Germany.
The response of metal nanostructures to optical excitation leads to localized surface plasmon (LSP) generation with nanoscale field confinement driving applications in, for example, quantum optics and nanophotonics. Field sampling in the terahertz domain has had a tremendous impact on the ability to trace such collective excitations. Here, we extend such capabilities and introduce direct sampling of LSPs in a more relevant petahertz domain.
View Article and Find Full Text PDFProc Natl Acad Sci U S A
January 2024
Institute for Quantum Information, Rheinish-Westfälisch Technische Hochschule (RWTH) Aachen University, 52056 Aachen, Germany.
We develop a photonic description of short, one-dimensional electromagnetic pulses, specifically in the language of electrical transmission lines. Current practice in quantum technology, using arbitrary waveform generators, can readily produce very short, few-cycle pulses in a very-low-noise, low-temperature setting. We argue that these systems attain the limit of producing pure coherent quantum states, in which the vacuum has been displaced for a short time, and therefore over a short spatial extent.
View Article and Find Full Text PDFJ Phys Chem A
November 2023
Department of Chemical Sciences, Indian Institute of Science Education and Research Kolkata, Kolkata, West Bengal 741246, India.
We have performed a coupled electron-nuclear dynamics study of H molecular ions under the influence of an intense few-cycle 4.5 fs laser pulse with an intensity of 4 × 10 W/cm and a central wavelength of 750 nm. Both quantum and classical dynamical methods are employed in the exact similar initial conditions with the aim of head-to-head comparison of two methodologies.
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