We demonstrate ultrafast tuning of a plasmonic spectral filter at terahertz (THz) frequencies. The device is made of periodically spaced gold crosses deposited on the surface of an undoped silicon wafer in which transient free carriers can be optically injected with a femtosecond resonant pulse. We demonstrate the concept by measuring the transmission spectrum of a notch filter using time-domain THz spectroscopy. Proper synchronization of the THz probe and visible excitation pulses leads to an enhanced transmission at the resonance by more than two orders of magnitude. Finite-difference time-domain simulations, which are in agreement with the experimental results, show that the underlying mechanisms responsible for the resonance blueshift and linewidth broadening can be attributed to the photoinduced change in dielectric properties of the substrate. This is supported by the numerically simulated field distribution and reflection/transmission coefficients. The device can be used in future pulse shaping and ultrafast switching experiments.
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http://dx.doi.org/10.1364/OE.395508 | DOI Listing |
ACS Appl Mater Interfaces
January 2025
College of Optical, Mechanical and Electrical Engineering, Zhejiang A&F University, Lin'an 311300, China.
As a member of the chalcogenide family, NiSe exhibits a direct bandgap of 1.74 eV, making it a promising candidate for nonlinear optical devices. However, its potential in the near-infrared region of the telecommunication band has not been fully explored.
View Article and Find Full Text PDFNanomaterials (Basel)
December 2024
College of Science, Inner Mongolia University of Technology, Hohhot 010051, China.
Relaxor ferroelectric film capacitors exhibit high power density with ultra-fast charge and discharge rates, making them highly advantageous for consumer electronics and advanced pulse power supplies. The Aurivillius-phase bismuth layered ferroelectric films can effectively achieve a high breakdown electric field due to their unique insulating layer ((BiO) layer)). However, designing and fabricating Aurivillius-phase bismuth layer relaxor ferroelectric films with optimal energy storage characteristics is challenging due to their inherently stable ferroelectric properties.
View Article and Find Full Text PDFACS Nano
December 2024
School of Materials Science and Engineering, Shanghai Jiao Tong University, Shanghai 200240, China.
Ultrafast thermal switches are pivotal for managing heat generated in advanced solid-state applications, including high-speed chiplets, thermo-optical modulators, and on-chip lasers. However, conventional phonon-based switches cannot meet the demand for picosecond-level response times, and existing near-field radiative thermal switches face challenges in efficiently modulating heat transfer across vacuum gaps. To overcome these limitations, we propose an ultrafast thermal switch design based on pump-driven transient polaritons in asymmetric terminals.
View Article and Find Full Text PDFCell Rep Phys Sci
December 2024
Centro Singular de Investigación en Química Biolóxica e Materiais Moleculares (CiQUS), Departamento de Física de Partículas, Universidade de Santiago de Compostela, 15782 Santiago de Compostela, Spain.
Porphyrinic metal-organic frameworks (MOFs) offer high surface areas and tunable catalytic and optoelectronic properties, making them versatile candidates for applications in phototherapy, drug delivery, photocatalysis, electronics, and energy storage. However, a key challenge for industrial integration is the rapid, cost-effective production of suitable sizes. This study introduces Zr(IV) alkoxides as metal precursors, achieving ultrafast (∼minutes) and high-yield (>90%) synthesis of three well-known Zr-based porphyrinic MOF nanocrystals: MOF-525, PCN-224, and PCN-222, each with distinct topologies.
View Article and Find Full Text PDFJ Synchrotron Radiat
January 2025
Shanghai Advanced Research Institute, Chinese Academy of Sciences, Shanghai 201204, People's Republic of China.
The combination of reversible angular dispersion-induced microbunching (ADM) and the rapid damping storage ring provides a storage-ring-based light source with the capability to produce longitudinal coherent radiation with a high repetition rate. This paper presents a prototype design for a test facility based on the study by Jiang et al. [Sci.
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