Increasing ellipticity usually suppresses the recollision probability drastically. In contrast, we report on a recollision channel with large return energy and a substantial probability, regardless of the ellipticity. The laser envelope plays a dominant role in the energy gained by the electron, and in the conditions under which the electron comes back to the core. We show that this recollision channel efficiently triggers various nonlinear and nonperturbative phenomena-such as multiple ionization-with an elliptically polarized pulse.
Download full-text PDF |
Source |
---|---|
http://dx.doi.org/10.1103/PhysRevLett.124.253203 | DOI Listing |
Phys Rev Lett
December 2024
Institute for Structure and Function and Department of Physics and Chongqing Key Laboratory for Strongly Coupled Physics, Chongqing University, Chongqing 400044, People's Republic of China and Center of Quantum Materials and Devices, Chongqing University, Chongqing 400044, People's Republic of China.
Phys Rev Lett
December 2024
School of Physics and Electronics, Hunan University, Changsha 410082, China.
Electron-hole exchange interaction in two-dimensional transition metal dichalcogenides is extremely strong due to the dimension reduction, which promises valley-superposed excitonic states with linearly polarized optical emissions. However, strong circular polarization reflecting valley-polarized excitonic states is commonly observed in helicity-resolved optical experiments. Here, we present a non-Hermitian theory of valley excitons by incorporating optical pumping and intrinsic decay, which unveils an anomalous valley-polarized excitonic state with elliptically polarized optical emission.
View Article and Find Full Text PDFScience
December 2024
Center for Complex Particle Systems (COMPASS), University of Michigan, Ann Arbor, MI, USA.
Planck's law ignores but does not prohibit black-body radiation (BBR) from being circularly polarized. BBR from nanostructured filaments with twisted geometry from nanocarbon or metal has strong ellipticity from 500 to 3000 nanometers. The submicrometer-scale chirality of these filaments satisfies the dimensionality requirements imposed by fluctuation-dissipation theorem and requires symmetry breaking in absorptivity and emissivity according to Kirchhoff's law.
View Article and Find Full Text PDFAdv Mater
December 2024
Shaanxi Joint Lab of Graphene, State Key Lab Incubation Base of Photoelectric Technology and Functional Materials, International Collaborative Center on Photoelectric Technology and Nano Functional Materials, Institute of Photonics & Photon-Technology, Northwest University, Xi'an, 710069, P. R. China.
Bulk photovoltaic effect (BPVE) can break the Shockley-Queisser limit by leveraging the inherent asymmetry of crystal lattice without a junction. However, this effect is mainly confined to UV-vis spectrum due to the wide-bandgap nature of traditional ferroelectric materials, thereby limiting the exploration of the infrared light-driven efficient BPVE. Herein, giant two-photon absorption (TPA) driven BPVE is uncovered from visible to infrared in ferroelectric α-InSe utilizing wavelength-tunable terahertz (THz) emission spectroscopy.
View Article and Find Full Text PDFJ Chem Phys
December 2024
State Key Laboratory of Precision Spectroscopy, School of Physics and Electronic Science, East China Normal University, Shanghai 200241, China.
Using ion-ion coincidence measurements, we experimentally investigate the dissociative triple ionization of argon dimers in relative phase controlled elliptically polarized two-color femtosecond laser fields. By examining the kinetic energy release-dependent momentum angular distribution of the ejected ionic fragments, two distinct pathways, each associated with different intermediates, are identified. Control over the emission directions of the ionic fragments is achieved by varying the relative phase of the elliptical two-color laser fields.
View Article and Find Full Text PDFEnter search terms and have AI summaries delivered each week - change queries or unsubscribe any time!