A novel coordination tailoring top-down delamination strategy involving the controllable partial disassembly of water-labile 3D MOFs has been explored to fabricate ultrathin 2D MOF nanosheets, and it exhibits many advantages such as green, convenience and high efficiency. Accordingly, 2D ultrathin MOF nanosheets with a two-fold interpenetrated architecture have been rapidly obtained from a 3D pillar-layered MOF, and they show distinguished fluorescence responses to different solvents.

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http://dx.doi.org/10.1039/d0nr02956dDOI Listing

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