We report the synthesis, crystal and band structures, and transport properties of organic conductor κ-(ET)Cu[Au(CN)]Cl [ET = bis(ethylenedithio)tetrathiafulvalene], which has a triangular spin-lattice ( = /) composed of (ET) dimers and polyanions with no disorder. The anisotropy of triangular lattice '/ = 1.19 and physical properties indicate that this material is the first ET-based quantum-spin-liquid candidate having a nearly regular triangular lattice with a disorder-free anion.
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| http://dx.doi.org/10.1021/acs.inorgchem.0c00880 | DOI Listing |
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