A switchable metasurface composed of plasmonic split ring resonators and a dye-doped liquid crystal is developed. The transmission of the metasurface in the infrared spectral range can be changed by illuminating the dye-doped liquid crystal with light in the visible spectral range. The effect is particularly efficient in the case of hybrid alignment of the liquid crystal, i. e. alignment of the director perpendicular to the surface on one substrate and parallel alignment on the counter substrate. This all-optical switching effect can be attributed to the behavior described in earlier works as colossal optical nonlinearity or surface-induced nonlinear optical effect.
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http://dx.doi.org/10.1364/OE.383877 | DOI Listing |
J Phys Chem B
December 2024
School of Energy and Power Engineering, Northeast Electric Power University, Jilin 132012, China.
When water is confined in a nanochannel, its thermodynamic and kinetic properties change dramatically compared to the macroscale. To investigate these phenomena, we conducted nonequilibrium molecular dynamics simulations on the heat transfer in copper-water nanochannels with lengths ranging from 12 to 20 nm in the absence and presence of an electric field. The results indicate that in the absence of an electric field ( = 12-20 nm), the binding force between water molecules in the 20 nm nanochannel is the weakest, facilitating thermal motion in the liquid phase.
View Article and Find Full Text PDFPhys Rev Lett
December 2024
QCD Labs, QTF Centre of Excellence, Department of Applied Physics, Aalto University, P.O. Box 13500, FI-00076 Aalto, Finland.
Ordered media often support vortex structures with intriguing topological properties. Here, we investigate non-Abelian vortices in tetrahedral order using the mathematical formalism of colored links. Due to the generality of our methods, the results apply to all physical systems governed by tetrahedral order, such as the cyclic phase of spin-2 Bose-Einstein condensates and the tetrahedratic phase of bent-core nematic liquid crystals.
View Article and Find Full Text PDFPhys Rev Lett
December 2024
Wuhan National High Magnetic Field Center and School of Physics, Huazhong University of Science and Technology, 430074 Wuhan, China.
The frustrated honeycomb spin model can stabilize a subextensively degenerate spiral spin liquid with nontrivial topological excitations and defects, but its material realization remains rare. Here, we report the experimental realization of this model in the structurally disorder-free compound GdZnPO. Using a single-crystal sample, we find that spin-7/2 rare-earth Gd^{3+} ions form a honeycomb lattice with dominant second-nearest-neighbor antiferromagnetic and first-nearest-neighbor ferromagnetic couplings, along with easy-plane single-site anisotropy.
View Article and Find Full Text PDFPhys Rev Lett
December 2024
Departament de Física, Campus Nord B4-B5, Universitat Politècnica de Catalunya, E-08034 Barcelona, Spain.
We predict that ultracold bosonic dipolar gases, confined within a multilayer geometry, may undergo self-assembling processes, leading to the formation of chain gases and solids. These dipolar chains, with dipoles aligned across different layers, emerge at low densities and resemble phases observed in liquid crystals, such as nematic and smectic phases. We calculate the phase diagram using quantum Monte Carlo methods, introducing a newly devised trial wave function designed for describing the chain gas, where dipoles from different layers form chains without in-plane long-range order.
View Article and Find Full Text PDFAngew Chem Int Ed Engl
December 2024
Shanghai Jiaotong University: Shanghai Jiao Tong University, School of Chemistry and Chemical Engineeringg, Dongchuan Road, Num 800, 200092, Shanghai, CHINA.
Circularly polarized luminescence (CPL) film attracted considerable attention in information storage and encryption, three-dimensional display, and chiral recognition. However, due to the limited molecular mobility within thin film, achieving a high asymmetry factor and non-contact modulation of CPL remain challenging. In this work, color-switchable homochiral CPL films with high luminescence asymmetry factor (glum~0.
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