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Spin-crossover in an organic-inorganic hybrid perovskite. | LitMetric
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Spin-crossover in an organic-inorganic hybrid perovskite.

Wei-Wei Wu Si-Guo Wu Yan-Cong Chen Guo-Zhang Huang Bang-Heng Lyu Zhao-Ping Ni Ming-Liang Tong

Chem Commun (Camb)

Key Laboratory of Bioinorganic and Synthetic Chemistry of Ministry of Education, School of Chemistry, Sun Yat-Sen University, Guangzhou, 510275, P. R. China.

Published: April 2020

The first spin-crossover (SCO) complex with an organic-inorganic hybrid perovskite structure (PPN)[Fe{Au(CN)}] (1) is reported, which displays three-step SCO behaviour. The light-induced excited spin-state trapping measurement gives T = 134 K for a three-dimensional FeL-type (L = bis-monodentate ligand) SCO complex. Moreover, spin-state dependent fluorescence is observed in 1.

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http://dx.doi.org/10.1039/d0cc00992jDOI Listing

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