Effect of preparation and reaction conditions on the performance of In/H-Beta for selective catalytic reduction of NO with CH.

Chemosphere

Shenzhen Key Laboratory of Organic Pollution Prevention and Control, Environmental Science and Engineering Research Center, Harbin Institute of Technology (Shenzhen), Shenzhen, 518055, PR China. Electronic address:

Published: August 2020

In/H-Beta catalyst was prepared by optimizing the support, concentration of ion exchange liquid and calcination temperature to investigate the effects of synthesis conditions on catalytic activity of selective catalytic reduction of NO with CH. The results showed that the In/H-Beta catalyst exhibited the superior activity when concentration of exchange liquid was 0.033 M and calcination temperature was 500 °C, the NO removal ratio could reach 97.6%. In addition, reaction conditions could affect the catalytic performance. When O concentration was 10%, CH:NO ratio was no less than one, space velocity was lower than 23600 h and NO initial concentration was no more than 700 ppm, In/H-Beta could exhibit superior catalytic activity. Moreover, the catalytic performances of In/H-Beta catalysts were discussed after enduring HO or/and SO. This novel strategy could open the door for selective catalytic reduction of NO with CH.

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http://dx.doi.org/10.1016/j.chemosphere.2020.126458DOI Listing

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