We experimentally demonstrate stimulated four-wave mixing in two linearly uncoupled integrated $ {{\rm Si}_3}{{\rm N}_4} $SiN micro-resonators. In our structure, the resonance combs of each resonator can be tuned independently, with the energy transfer from one resonator to the other occurring in the presence of a nonlinear interaction. This method allows flexible and efficient on-chip control of the nonlinear interaction, and is readily applicable to other third-order nonlinear phenomena.
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Multiple coherent radiations are achieved in a water-3-aminopropanol (3AP) mixed solution through cascaded four-wave mixing (C-FWM) and cascaded Stokes (C-Stokes) processes, both driven by stimulated Raman scattering (SRS) in this work. The O-H vibration peak from water is replaced by the emergence of the -NH symmetric stretching Raman peaks from 3AP, with intensity approaching that of the -CH symmetric stretching peak. The dual-wavelength SRS signals for the -NH and -CH stretching vibrations have a relatively small frequency interval of about 400 cm (16 nm).
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View Article and Find Full Text PDFLinear and nonlinear optics in composite systems: From diagrammatic modeling to applications.
J Chem Phys
June 2024
Université Paris-Saclay, CNRS, Institut de Chimie Physique, UMR 8000, 91405 Orsay, France.
A bipartite system is defined as two microscopic entities being able to exchange energy. When excited by light, the complete optical response functions at first (polarizabilities) and second orders (first hyperpolarizabilities) of such a system are determined using the diagrammatic theory of optics. The generality of the method is ensured by the free choice of light-matter and matter-matter interaction Hamiltonians and by the arbitrary number of quanta involved in the energy exchange.
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