We perform a global sensitivity analysis of the binding energy and the charge radius of the nucleus ^{16}O to identify the most influential low-energy constants in the next-to-next-to-leading order chiral Hamiltonian with two- and three-nucleon forces. For this purpose, we develop a subspace-projected coupled-cluster method using eigenvector continuation [Frame D. et al., Phys. Rev. Lett. 121, 032501 (2018)PRLTAO0031-900710.1103/PhysRevLett.121.032501]. With this method, we compute the binding energy and charge radius of ^{16}O at more than 10^{6} different values of the 16 low-energy constants in one hour on a standard laptop computer. For relatively small subspace projections, the root-mean-square error is about 1% compared to full-space coupled-cluster results. We find that 58(1)% of the variance in energy can be apportioned to a single contact term in the ^{3}S_{1} wave, whereas the radius depends sensitively on several low-energy constants and their higher-order correlations. The results identify the most important parameters for describing nuclear saturation and help prioritize efforts for uncertainty reduction of theoretical predictions. The achieved acceleration opens up an array of computational statistics analyses of the underlying description of the strong nuclear interaction in nuclei across the Segrè chart.
Download full-text PDF |
Source |
---|---|
http://dx.doi.org/10.1103/PhysRevLett.123.252501 | DOI Listing |
EES Catal
December 2024
Department of Chemical Engineering, Delft University of Technology 2629 HZ Delft The Netherlands
Electrochemical CO reduction offers a promising method of converting renewable electrical energy into valuable hydrocarbon compounds vital to hard-to-abate sectors. Significant progress has been made on the lab scale, but scale-up demonstrations remain limited. Because of the low energy efficiency of CO reduction, we suspect that significant thermal gradients may develop in industrially relevant dimensions.
View Article and Find Full Text PDFPolymers (Basel)
December 2024
A.M. Butlerov Chemical Institute, Kazan Federal University, Kazan 420008, Russia.
This article is devoted to the development of a new method for the synthesis of magnetic cobalt boride nanoparticles using a low-energy approach. The obtained nanoparticles were used to create composite materials based on industrial thermoplastic ABS. The effect of different concentrations of nanoparticles on the physical, mechanical, magnetic, and dielectric properties of composite materials was studied.
View Article and Find Full Text PDFAdv Mater
December 2024
Beijing National Laboratory for Molecular Sciences, CAS Key Laboratory of Organic Solids and State Key Laboratory of Polymer Physics and Chemistry, Institute of Chemistry, Chinese Academy of Sciences, Beijing, 100190, China.
Highly efficient nonfullerene acceptors (NFAs) for organic solar cells (OSCs) with low energy loss (E) and favorable morphology are critical for breaking the efficiency bottleneck and achieving commercial applications of OSCs. In this work, quinoxaline-based NFAs are designed and synthesized using a synergistic isomerization and bromination approach. The π-expanded quinoxaline-fused core exhibits different bromination sites for isomeric NFAs, namely AQx-21 and AQx-22.
View Article and Find Full Text PDFJ Mass Spectrom
January 2025
Research Center for Energy and Environmental Materials, National Institute for Materials Science, Tsukuba, Ibaraki, Japan.
A possible TOF-SIMS analysis of surface phase transitions has recently been proposed for limited cases such as polymers and ionic liquids. In the present study, we have extended this analysis to quench-condensed noble gas films. The newly developed cryogenic TOF-SIMS allowed both measurements of TOF-SIMS below 4 K, and low-energy ion scattering spectroscopy that is used to prepare a clean surface.
View Article and Find Full Text PDFJ Nutr Sci
December 2024
Faculty of Health & Medical Sciences, University of Surrey, Guildford, United Kingdom of Great Britain and Northern Ireland.
Weight loss results in obligatory reductions in energy expenditure (EE) due to loss of metabolically active fat-free mass (FFM). This is accompanied by adaptive reductions (i.e.
View Article and Find Full Text PDFEnter search terms and have AI summaries delivered each week - change queries or unsubscribe any time!