Quantum Beat between Sunlight and Single Photons.

Nano Lett

Shanghai Branch, Department of Modern Physics and National Laboratory for Physical Sciences at Microscale , University of Science and Technology of China, Shanghai 201315 , China.

Published: January 2020

We demonstrate fourth-order quantum beat between sunlight and single photons from a quantum dot. With a fast time-resolved detection system, we observed high-visibility quantum beat between the independent photons of different frequencies from the two astronomically separated light sources. The temporal dynamics of the beat oscillation indicate the coherent behavior of the interfering photons, and the raw visibility of two-photon interference shows violation of the classical limit with a frequency mismatch of three-times the line width.

Download full-text PDF

Source
http://dx.doi.org/10.1021/acs.nanolett.9b03512DOI Listing

Publication Analysis

Top Keywords

quantum beat
12
beat sunlight
8
sunlight single
8
single photons
8
quantum
4
photons
4
photons demonstrate
4
demonstrate fourth-order
4
fourth-order quantum
4
photons quantum
4

Similar Publications

Two-dimensional electronic spectroscopy (2DES) has high spectral resolution and is a useful tool for studying atomic dynamics. In this paper, we show a smallest unit of electromagnetically induced transparency (EIT) for 2DES, i.e.

View Article and Find Full Text PDF

Vibronic coherent quantum beat in four-layer platinum carbonyl cluster.

J Chem Phys

November 2024

College of Chemistry and Molecular Engineering, Beijing National Laboratory for Molecular Sciences, Peking University, Beijing 100871, People's Republic of China.

Vibronic coherence has been studied for years, but direct comparisons between the rich experimental features and theory remain rare. In this work, we investigate the vibronic coherent quantum beat of a four-layer platinum carbonyl cluster [Pt3(CO)6]42- in a solution utilizing femtosecond vis-pump/vis-probe transient absorption spectroscopy. By varying the excitational wavelength, quantum beats coupled to either the electronic ground state or the excited state are selectively prepared.

View Article and Find Full Text PDF

Revealing and Manipulating Hidden Fine-Structure Coherence of Bright Excitons in CsPbI Perovskite Quantum Dots.

Nano Lett

November 2024

State Key Laboratory of Molecular Reaction Dynamics, Dalian Institute of Chemical Physics, Chinese Academy of Sciences, Dalian, Liaoning 116023, China.

Observation and understanding of fine-structure splitting of bright excitons in lead halide perovskite quantum dots (QDs) are crucial to their emerging applications in quantum light sources and exciton coherence manipulation. Recent studies demonstrate that ensemble-level polarization-resolved transient absorption spectroscopy can reveal the quantum beats arising from the coherence between two fine-structure levels. Here we report the observation of an extra fine-structure quantum coherence hidden in previous studies by using cryo-magnetic quantum beat spectroscopy.

View Article and Find Full Text PDF

Quadrupole Coupling of Circular Rydberg Qubits to Inner Shell Excitations.

Phys Rev Lett

September 2024

5. Physikalisches Institut and Center for Integrated Quantum Science and Technology, Universität Stuttgart, Pfaffenwaldring 57, 70569 Stuttgart, Germany.

Article Synopsis
  • Divalent atoms have potential for improved control in quantum simulation and computing due to a second valence electron, with circular Rydberg atoms being especially promising for avoiding autoionization.
  • A specific experiment used electric quadrupole coupling between a metastable 4D_{3/2} level and a high-n circular Rydberg qubit in ^{88}Sr atoms, measuring a small differential level shift with advanced interferometry techniques.
  • The study demonstrated effective qubit coherence maintenance despite continuous photon scattering, opening new avenues for laser cooling and further manipulation of Rydberg atoms in quantum computing.
View Article and Find Full Text PDF

Want AI Summaries of new PubMed Abstracts delivered to your In-box?

Enter search terms and have AI summaries delivered each week - change queries or unsubscribe any time!