Transient electronics have dramatically changed inner-body therapy in health care. They stand out because of their harmless dissolution in the human body with no lingering electronic trash. However, high-precision biomedical implants require programmable and serial remedy operations, and controlling the whole-device destruction is not proactive and precise. Thus, a novel biotriggered and temperature-controlled transient electronics fabrication method using elastin-like polypeptides (ELPs) as triggers is proposed. Biocompatible ELPs simply mixed with trace silver nanowire (AgNW) can serve as the "switch" for the electronics to respond to local temperature changes in deionized water, exhibiting an agile response time. A ratio gradient experiment of the ELPs and AgNW shows that more programmable and precise transience properties (initial resistance, ready time, response time, and stable resistance) can be achieved by using a designated proportion. Further, we validated that the 3D-printing-based ELP-triggering transient electronics fabrication method is very simple yet effective for preparing transient wireless charging LEDs. Transient devices comprising ELPs-AgNW and PLGA-Ag respond within 160 s below 10 °C and degrade within a certain period.
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http://dx.doi.org/10.1021/acsami.9b14798 | DOI Listing |
Soft Matter
March 2025
Institute of Electronic Structure & Laser, FORTH, Heraklion, 70013, Greece.
The cage concept, a central microscopic mechanism for glassy dynamics, has been utilized in concentrated colloidal suspensions to describe a number of phenomena. Here, we probe the evolution of cage formation and shear elasticity with increasing volume fraction in hard sphere suspensions, with emphasis on the short-time dynamics. To this end, we utilize linear viscoelastic (LVE) measurements, by means of conventional rotational rheometers and a home-made HF piezo-rheometer, to probe the dynamic response over a broad range of volume fractions up to the very dense glassy regime in proximity to random close packing.
View Article and Find Full Text PDFNano Lett
March 2025
State Key Laboratory of Integrated Optoelectronics, College of Electronic Science and Engineering, Jilin University, Changchun 130012, China.
Inserting intermediate layers in transition metal dichalcogenide heterostructures (TMD HSs) has become an efficient approach to modulating interlayer charge transfer rates. However, it could not only modify the distance of charge transfer but also potentially alter the interlayer coupling strength within HSs, which would profoundly influence the charge transfer rate in the opposite direction. Here, to gain insight into the dual roles of inserted intermediate layers in multilayer TMD HSs, MoS-L WSe-MoSe ( = 1-3) HSs were designed and systemically investigated.
View Article and Find Full Text PDFAngew Chem Int Ed Engl
March 2025
Nanjing Tech University, Institute of Advanced Materials (IAM), 5 Xinmofan Road, 210009, Nanjing, CHINA.
The development of small molecular dyes excitable in the second near-infrared window (NIR-II, 1000~1700 nm) is crucial for deep-tissue penetration and maximum permissible exposure in cancer photothermal theranostics. Herein, we employed a dendrimer engineering strategy to develop the boron difluoride formazanate (BDF) dye BDF-8OMe for photoacoustic imaging-mediated NIR-II photothermal therapy. BDF-8OMe, characterized by an increased molecular branching degree and extended π-conjugation, exhibited broad absorbance peaked at 905 nm, with the absorption tail extending to 1300 nm.
View Article and Find Full Text PDFACS Appl Mater Interfaces
March 2025
Extreme Materials Research Center, Korea Institute of Science and Technology, Seoul 02792, Republic of Korea.
Transient electronics, designed to degrade after a defined period, are ideal for biomedical implants that eliminate the need for secondary removal surgeries and contribute to sustainable electronics by leaving no electronic waste. While significant progress has been made in developing semiconductors, electrodes, and substrates, dielectric layers for bioapplicable transient electronics that combine flexibility, self-healing capabilities, and high dielectric constants (high-k) remain underexplored. This study introduces urea-linked polycaprolactone (PCL-IU)/ionic liquid (IL) hybrids as dielectric materials.
View Article and Find Full Text PDFClin Nutr
February 2025
Department of Clinical Research, Acute CAG, Copenhagen University Hospital, Amager and Hvidovre, Denmark. Electronic address:
Background And Aims: Anorexia of aging is prevalent and constitutes a significant factor in the onset of malnutrition with limited effective interventions. Cannabis-based medicine (CBM) with delta-9-tetrahydrocannabinol (THC) and cannabidiol (CBD) may have orexigenic properties in older patients with poor appetite. However, current evidence is insufficient regarding the impact of CBM in older patients with poor appetite.
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