We study the thermoelectric properties of a Kramers pair of helical edge states of the quantum spin Hall effect coupled to a nanomagnet with a component of the magnetization perpendicular to the direction of the spin-orbit interaction of the host. We show that the transmission function of this structure has the desired qualities for optimal thermoelectric performance in the quantum coherent regime. For a single magnetic domain, there is a power generation close to the optimal bound. In a configuration with two magnetic domains with different orientations, pronounced peaks in the transmission functions and resonances lead to a high figure of merit. We provide estimates for the fabrication of this device with HgTe quantum-well topological insulators.
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http://dx.doi.org/10.1103/PhysRevLett.123.186801 | DOI Listing |
Adv Mater
January 2025
State Key Laboratory for Manufacturing Systems Engineering, Electronic Materials Research Laboratory, Key Laboratory of the Ministry of Education, School of Electronic Science and Engineering, Xi'an Jiaotong University, Xi'an, 710049, China.
Large low-field magnetoresistance (LFMR, < 1 T), related to the spin-disorder scattering or spin-polarized tunneling at boundaries of polycrystalline manganates, holds considerable promise for the development of low-power and ultrafast magnetic devices. However, achieving significant LFMR typically necessitates extremely low temperatures due to diminishing spin polarization as temperature rises. To address this challenge, one strategy involves incorporating Ruddlesden-Popper structures (ABO):AO, which are layered derivatives of perovskite structure capable of potentially inducing heightened magnetic fluctuations at higher temperatures.
View Article and Find Full Text PDFPhys Chem Chem Phys
January 2025
King Abdullah University of Science and Technology (KAUST), Physical Science and Engineering Division (PSE), Thuwal 23955-6900, Saudi Arabia.
Employing density functional theory for ground state quantum mechanical calculations and the non-equilibrium Green's function method for transport calculations, we investigate the potential of CdS, ZnS, CdZnS, and ZnCdS as tunnel barriers in magnetic tunnel junctions for spintronics. Based on the finding that the valence band edges of these semiconductors are dominated by p orbitals and the conduction band edges by s orbitals, we show that symmetry filtering of the Bloch states in magnetic tunnel junctions with Fe electrodes results in high tunneling magnetoresistances and high spin-polarized current (up to two orders of magnitude higher than in the case of the Fe/MgO/Fe magnetic tunnel junction).
View Article and Find Full Text PDFJ Phys Chem C Nanomater Interfaces
January 2025
Institute of General, Inorganic and Theoretical Chemistry, University of Innsbruck,Innrain 80-82, 6020 Innsbruck, Austria.
Cu-doped LaCu Mn O perovskites have been used as a model system for a joint experimental and theoretical assessment of the influence of the Cu doping level on the structural, electronic, and magnetic properties. The different Cu-doped phases LaCuMnO (LCM37), LaCuMnO (LCM55), and LaCuMnO (LCM73) including the respective Cu- and Mn-free benchmark materials LaCuO (LC) and LaMnO (LM) have been studied by magnetization measurements and electronic paramagnetic resonance. Ferromagnetic behavior was detected for pure LM and all Cu-doped perovskites, whereas antiferromagnetic behavior was revealed for LaCuO.
View Article and Find Full Text PDFJ Phys Chem C Nanomater Interfaces
January 2025
Instituto de Nanociencia y Materiales de Aragón (INMA), CSIC - Universidad de Zaragoza, Plaza San Francisco s/n, Zaragoza 50009, Spain.
A strategy toward the realization of a quantum spin processor involves the coupling of spin qubits and qudits to photons within superconducting resonators. To enable the realization of such hybrid architecture, here we first explore the design of a chip with multiple lumped-element LC superconducting resonators optimized for their coupling to distinct transitions of a vanadyl porphyrin electronuclear qudit. The controlled integration of the vanadyl qudit onto the superconducting device, both in terms of number and orientation, is then attained using the formation of nanosheets of a 2D framework built on the vanadyl qudit as a node.
View Article and Find Full Text PDFNano Lett
January 2025
University of Washington, Physics Department, Seattle, Washington 98105, United States.
The charge state of a quantum point defect in a solid-state host strongly determines its optical and spin characteristics. Consequently, techniques for controlling the charge state are required to realize technologies for quantum networking and sensing. In this work, we demonstrate the use of deep-ultraviolet (DUV) radiation to dynamically neutralize nitrogen- (NV) and silicon-vacancy (SiV) centers.
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