Improved long-wavelength transmission and supercontinuum (SC) generation is demonstrated by antireflective (AR) nanoimprinting and tapering of chalcogenide photonic crystal fibers (PCFs). Using a SC source input spanning from 1 to 4.2 μm, the total transmission of a 15 μm core diameter PCF was improved from ∼53% to ∼74% by nanoimprinting of AR structures on both input and output facets of the fiber. Through a combined effect of reduced reflection and redshifting of the spectrum to 5 μm, the relative transmission of light >3.5 μm in the same fiber was increased by 60.2%. Further extension of the spectrum to 8 μm was achieved using tapered fibers. The spectral broadening dynamics and output power were investigated using different taper parameters and pulse repetition rates.
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http://dx.doi.org/10.1364/OL.44.005505 | DOI Listing |
Nanotechnology
November 2023
Micro- and Nano-technology Research Center, State Key Laboratory for Manufacturing Systems Engineering, Xi'an Jiaotong University, Xi'an 710049, People's Republic of China.
Nanopatterning complex uneven surface of numerous functional devices to improve their performance is significantly appealing; however, it is extremely challenging. This study proposes a discretely-supported transfer nanoimprint technique to fabricate nanostructures on complex device surfaces containing multi-spatial frequencies. First, a discretely-supported nanoimprint template was designed based on the built energy criterion.
View Article and Find Full Text PDFRev Sci Instrum
March 2023
HighRI Optics, Inc., 5401 Broadway Ter 304, Oakland, California 94618, USA.
The ability to correlate optical hyperspectral mapping and high resolution topographic imaging is critically important to gain deep insight into the structure-function relationship of nanomaterial systems. Scanning near-field optical microscopy can achieve this goal, but at the cost of significant effort in probe fabrication and experimental expertise. To overcome these two limitations, we have developed a low-cost and high-throughput nanoimprinting technique to integrate a sharp pyramid structure on the end facet of a single-mode fiber that can be scanned with a simple tuning-fork technique.
View Article and Find Full Text PDFNano Lett
December 2022
School of Physical Science and Technology, ShanghaiTech University, Shanghai 201210, China.
Insufficient catalyst utilization, limited mass transport, and high ohmic resistance of the conventional membrane electrode assembly (MEA) lead to significant performance losses of proton exchange membrane water electrolysis (PEMWE). Herein we propose a novel ordered MEA based on anode with a 3D membrane/catalytic layer (CL) interface and gradient tapered arrays by the nanoimprinting method, confirmed by energy dispersive spectroscopy. Benefiting from the maximized triple-phase interface, rapid mass transport, and gradient CL by overall design, such an ordered structure with Ir loading of 0.
View Article and Find Full Text PDFImproved long-wavelength transmission and supercontinuum (SC) generation is demonstrated by antireflective (AR) nanoimprinting and tapering of chalcogenide photonic crystal fibers (PCFs). Using a SC source input spanning from 1 to 4.2 μm, the total transmission of a 15 μm core diameter PCF was improved from ∼53% to ∼74% by nanoimprinting of AR structures on both input and output facets of the fiber.
View Article and Find Full Text PDFThe common complex architecture constitutes the major bottleneck of optical absorber operating on broadband spectrum. Here we demonstrate a super absorber consisting of tapered dielectric nanostructure coated with a thin-layer of non-noble metal chromium on flexible poly(ethylene terephthalate) substrate. The proposed device yields double-sided, omnidirectional, and polarization-independent absorption over the entire visible spectrum with an average efficiency more than 90% at normal incidence, and 80% at a tilt incident angle of 60°.
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