A nearly single cycle intense terahertz (THz) pulse with peak electric and magnetic fields of 0.5 MV/cm and 0.16 T, respectively, excites both modes of spin resonances in the weak antiferromagnet FeBO_{3}. The high frequency quasiantiferromagnetic mode is excited resonantly and its amplitude scales linearly with the strength of the THz magnetic field, whereas the low frequency quasiferromagnetic mode is excited via a nonlinear mechanism that scales quadratically with the strength of the THz electric field and can be regarded as a THz inverse Cotton-Mouton effect. THz optomagnetism is shown to be more energy efficient than similar effects reported previously for the near-infrared spectral range.
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http://dx.doi.org/10.1103/PhysRevLett.123.157202 | DOI Listing |
J Phys Chem A
January 2025
Institute of Nanoscience and Engineering, Henan University, Kaifeng, Henan 475004, China.
With the rapid development of thermally activated delayed fluorescence (TADF) materials, achieving efficient reverse intersystem crossing (RISC) to mitigate triplet-triplet annihilation has emerged as a prominent research focus. This study investigates five derivative molecules, featuring varied bridging atoms/groups (O, S, Se, -CH-), designed from the reported TADF molecule with through-space charge transfer (TSCT) properties. Utilizing time-dependent density functional theory coupled with a PCM solution model, their excited state behaviors were simulated in a toluene environment.
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View Article and Find Full Text PDFPhys Rev Lett
December 2024
Radboud University Nijmegen, Institute for Molecules and Materials, 6525 AJ, Nijmegen, The Netherlands.
Resonant pumping of the electronic f-f transitions in the orbital multiplet of dysprosium ions (Dy^{3+}) in a complex perovskite DyFeO_{3} is shown to impulsively launch THz lattice dynamics corresponding to the B_{2g} phonon mode, which is dominanted by the motion of Dy^{3+} ions. The findings, supported by symmetry analysis and density-functional theory calculations, not only provide a novel route for highly selective excitation of the rare-earth crystal lattices but also establish important relationships between the symmetry of the electronic and lattice excitations in complex oxides.
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Department of Physics, 104 Davey Lab, Pennsylvania State University, University Park, Pennsylvania 16802, USA.
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State Key Laboratory of Extreme Photonics and Instrumentations, Centre for Optical and Electromagnetic Research, College of Optical Science and Engineering, International Research Center for Advanced Photonics, Zhejiang University, Hangzhou 310058, China.
Multichannel imaging in the second near-infrared (NIR-II) window offers vital and comprehensive information for complex surgical environments, yet a simple, high-quality, video-rate multichannel imaging method with low safety risk remains to be proposed. Centered at the superior NIR-IIx window of 1400-1500 nm, triple-channel imaging coordinated with 1000-1100 and 1700-1880 nm (NIR-IIc) achieves exceptional clarity and an impressive signal-to-crosstalk ratio as high as 22.10.
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