Indistinguishable single photon generation at telecom wavelengths from solid-state quantum emitters remains a significant challenge to scalable quantum information processing. Here we demonstrate efficient generation of "indistinguishable" single photons directly in the telecom O-band from aryl-functionalized carbon nanotubes by overcoming the emitter quantum decoherence with plasmonic nanocavities. With an unprecedented single-photon spontaneous emission time down to 10 ps (from initially 0.7 ns) generated in the coupling scheme, we show a two-photon interference visibility at 4 K reaching up to 0.79, even without applying post selection. Cavity-enhanced quantum yields up to 74% and Purcell factors up to 415 are achieved with single-photon purities up to 99%. Our results establish the capability to fabricate fiber-based photonic devices for quantum information technology with coherent properties that can enable quantum logic.
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http://dx.doi.org/10.1021/acs.nanolett.9b04069 | DOI Listing |
Nano Lett
January 2025
State Key Laboratory for Mesoscopic Physics and Frontiers Science Center for Nano-optoelectronics, School of Physics, Peking University, 100871 Beijing, China.
ACS Photonics
December 2024
School of Physics and Astronomy, University of Birmingham, Birmingham B15 2TT, U.K.
Tightly confined plasmons in metal nanogaps are highly sensitive to surface inhomogeneities and defects due to the nanoscale optical confinement, but tracking and monitoring their location is hard. Here, we probe a 1-D extended nanocavity using a plasmonic silver nanowire (AgNW) on mirror geometry. Morphological changes inside the nanocavity are induced locally using optical excitation and probed locally through simultaneous measurements of surface enhanced Raman scattering (SERS) and dark-field spectroscopy.
View Article and Find Full Text PDFSci Adv
December 2024
Department of Electrical and Computer Engineering, Boston University, Boston, MA 02215, USA.
Most molecules and dielectric materials have characteristic bond vibrations or phonon modes in the mid-infrared regime. However, infrared absorption spectroscopy lacks the sensitivity for detecting trace analytes due to the low quantum efficiency of infrared sensors. Here, we report mid-infrared photothermal plasmonic scattering (MIP-PS) spectroscopy to push the infrared detection limit toward nearly a hundred molecules in a plasmonic nanocavity.
View Article and Find Full Text PDFJ Chem Phys
December 2024
Guangdong Provincial Key Laboratory of Optoelectronic Information Processing Chips and Systems, School of Microelectronics Science and Technology, Sun Yat-sen University, Zhuhai 519082, China.
The strong coupling between infrared photonic resonances and vibrational transitions of organic molecules is called vibrational strong coupling (VSC), which presents attractive prospects for modifying molecular chemical characteristics and behaviors. Currently, VSC studies suffer from limited bandwidth or enormous mode volumes. In addition, in certain instances, the absorption spectrum of VSC is weaker, thus impeding the effective monitoring of the VSC effect.
View Article and Find Full Text PDFNanophotonics
June 2024
Vienna Center for Quantum Science and Technology (VCQ), Faculty of Physics, University of Vienna, Boltzmanngasse 5, 1090 Vienna, Austria.
Polariton thermalization is a key process in achieving light-matter Bose-Einstein condensation, spanning from solid-state semiconductor microcavities at cryogenic temperatures to surface plasmon nanocavities with molecules at room temperature. Originated from the matter component of polariton states, the microscopic mechanisms of thermalization are closely tied to specific material properties. In this work, we investigate polariton thermalization in strongly-coupled molecular systems.
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