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Discovery and Biosynthesis of Neoenterocins Indicate a Skeleton Rearrangement of Enterocin. | LitMetric
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Discovery and Biosynthesis of Neoenterocins Indicate a Skeleton Rearrangement of Enterocin.

Liujuan Zheng Xiaodong Jiang Qingbo Zhang Yiguang Zhu Haibo Zhang Wenjun Zhang Kumar Saurav Jinsong Liu Changsheng Zhang

Org Lett

Key Laboratory of Tropical Marine Bio-resources and Ecology, Guangdong Key Laboratory of Marine Materia Medica, RNAM Center for Marine Microbiology, Institutions of South China Sea Ecology and Environmental Engineering , South China Sea Institute of Oceanology, Chinese Academy of Sciences , 164 West Xingang Road , Guangzhou 510301 , China.

Published: November 2019

Two polyketides neoenterocins A () and B (), featuring a neighboring dicarbonyl motif and a furan-containing 5/6 ring system, were isolated from the enterocin producer sp. SCSIO 11863. Heterologous expression, gene disruptions, and isotope feeding experiments indicated that and were derived from the enterocin biosynthetic gene cluster. However, was demonstrated as an artifact from enterocin via a unique skeleton rearrangement.

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http://dx.doi.org/10.1021/acs.orglett.9b03460DOI Listing

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