Characterization of aerosol chemical composition and the reconstruction of light extinction coefficients during winter in Wuhan, China.

Chemosphere

Environmental Chemistry and Technology Program, University of Wisconsin-Madison, 660 North Park Street, Madison, WI, 53706, USA. Electronic address:

Published: February 2020

To evaluate light extinction contributions of aerosol chemical constituents and their impacts on atmospheric visibility, the PM and its chemical components, light scattering (b) and absorption (b) were continuously measured in Wuhan from January to February 2018. The average of PM concentration, b and b were 96.5 ± 13.7 μg m, 564 ± 124 Mm and 44 ± 8 Mm during polluted days, respectively, which was about 2.0, 2.1 and 1.6 times higher than those of clean days, respectively. Compared with the clean days, the increase of the mass concentrations of SNA (SO, NO, NH) during polluted days was higher than those of organic (OC) and elemental (EC) carbon, indicated the increase of SNA was the main cause of air pollution. The PM concentration threshold was 66 μg m, corresponding to the visibility lower than 10 km. The revised Interagency Monitoring of Protected Visual Environments (IMPROVE) algorithm was used to reconstruct the light extinction coefficient (b) in Wuhan. The sum of light extinction coefficients of (NH)SO, NHNO and organic matter (OM) accounted for 70.5% and 83.9% of b during clean and polluted days, respectively. The backward trajectory and potential source contribution function (PSCF) analysis revealed that regional transport accounted for 55.6% of the total airflow, which originated from south, northwest and west of Wuhan. The increases of (NH)SO and NHNO concentrations, emitted from local vehicle exhaust and coal combustion, and their hygroscopic growth in ambient were the major causes of pollution in Wuhan.

Download full-text PDF

Source
http://dx.doi.org/10.1016/j.chemosphere.2019.125033DOI Listing

Publication Analysis

Top Keywords

light extinction
16
polluted days
12
aerosol chemical
8
extinction coefficients
8
clean days
8
nhso nhno
8
light
5
wuhan
5
days
5
characterization aerosol
4

Similar Publications

Recent studies have unveiled the deep sea as a rich biosphere, populated by species descended from shallow-water ancestors post-mass extinctions. Research on genomic evolution and microbial symbiosis has shed light on how these species thrive in extreme deep-sea conditions. However, early adaptation stages, particularly the roles of conserved genes and symbiotic microbes, remain inadequately understood.

View Article and Find Full Text PDF

The elevated glutathione (GSH) level and hypoxia in tumor cells are two key obstacles to realizing the high performance of phototherapy. Herein, the electron-donating rotors are introduced to wings of electron-withdrawing pyrrolopyrrole cyanine (PPCy) to form donor-acceptor-donor structure -aggregates for amplified superoxide radical generation, GSH depletion, and photothermal action for hypoxic cancer phototherapy to tackle this challenge. Three PPCy photosensitizers (PPCy-H, PPCy-Br, and PPCy-TPE) produce hydroxyl radicals (•OH) and superoxide radicals (O) in hypoxia tumors exclusively as well as excellent photothermal performances under light irradiation.

View Article and Find Full Text PDF

Click beetle larvae from Cretaceous Burmese amber represent an ancient Gondwanan lineage.

Sci Rep

January 2025

Department of Geoinformatics, Faculty of Science, Palacky University, 17. listopadu 50, 77146, Olomouc, Czech Republic.

The click beetles (Elateridae) represent the major and well-known group of the polyphagan superfamily Elateroidea. Despite a relatively rich fossil record of Mesozoic Elateridae, only a few species are described from the Upper Cretaceous Burmese amber. Although Elateridae spend most of their lives as larvae, our knowledge on immature stages of this family is limited, which is especially valid for the fossils.

View Article and Find Full Text PDF

CRISPR/Cas12a with Universal crRNA for Indiscriminate Virus Detection.

Molecules

December 2024

Biotecnovo (Beijing) Co., Ltd., Room 801 Suit C Hengtai Center, Building 3 Gate, 18 North Feng Road, Fengtai District, Beijing 100176, China.

Viruses, known for causing widespread biological harm and even extinction, pose significant challenges to public health. Virus detection is crucial for accurate disease diagnosis and preventing the spread of infections. Recently, the outstanding analytical performance of CRISPR/Cas biosensors has shown great potential and they have been considered as augmenting methods for reverse-transcription polymerase chain reaction (RT-PCR), which was the gold standard for nucleic acid detection.

View Article and Find Full Text PDF

UV-vis spectroscopy is a workhorse in analytical chemistry that finds application in life science, organic synthesis, and energy technologies like photocatalysis. In its traditional implementation with cuvettes, it requires sample volumes in the milliliter range. Here, we show how nanofluidic scattering spectroscopy (NSS), which measures visible light scattered from a single nanochannel in a spectrally resolved way, can reduce this sample volume to the attoliter range for solute concentrations in the mM regime, which corresponds to as few as 10 probed molecules.

View Article and Find Full Text PDF

Want AI Summaries of new PubMed Abstracts delivered to your In-box?

Enter search terms and have AI summaries delivered each week - change queries or unsubscribe any time!