Degradation of phenol by coal-based carbon membrane integrating sulfate radicals-based advanced oxidation processes.

Ecotoxicol Environ Saf

State Key Laboratory of Fine Chemicals, Carbon Research Laboratory, School of Chemical Engineering, Dalian University of Technology, 2 Linggong Road, Dalian, 116024, China. Electronic address:

Published: December 2019

Phenol, as a representative organic pollutant in aquatic environments, has posed a serious threat to humans and ecosystem. In this work, a novel integration system combined coal-based carbon membrane with sulfate radicals-based advanced oxidation processes (SR-AOPs) was designed for degradation of phenol. The integrated system achieved 100% removal efficiency under the optimal condition (peroxydisulfate dosage is 0.2 g/L, at alkaline condition with 2 mL/min flow velocity). The quenching experiments revealed that the efficient removal of phenol by the integrated system were attributed to the co-existence of radical and nonradical mechanisms. This study proposes a green and efficient technique for the removal of phenol.

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http://dx.doi.org/10.1016/j.ecoenv.2019.109662DOI Listing

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