A deep understanding of the thermal properties of 2D materials is crucial to their implementation in electronic and optoelectronic devices. In this study, we investigated the macroscopic in-plane thermal conductivity (κ) and thermal interface conductance (g) of large-area (mm) thin film made from MoS nanoflakes via liquid exfoliation and deposited on Si/SiO substrate. We found κ and g to be 1.5 W/mK and 0.23 MW/mK, respectively. These values are much lower than those of single flakes. This difference shows the effects of interconnections between individual flakes on macroscopic thin film parameters. The properties of a Gaussian laser beam and statistical optothermal Raman mapping were used to obtain sample parameters and significantly improve measurement accuracy. This work demonstrates how to address crucial stability issues in light-sensitive materials and can be used to understand heat management in MoS and other 2D flake-based thin films.

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http://www.ncbi.nlm.nih.gov/pmc/articles/PMC6746815PMC
http://dx.doi.org/10.1038/s41598-019-49980-7DOI Listing

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