We present a nonlinear transfer matrix method for studying the second-harmonic generation (SHG) in nonperiodic metamaterial photonic superlattices. A large enhancement of up to 5 orders of magnitude in SHG efficiency was observed for superlattices made with a Cantor-like quasiperiodic assembly of a nonlinear material and a metamaterial. The enhancement was found to depend much more on the electric field amplitude along the structure because of self-similarity effects than on the amount of nonlinear material, which opens the way to design superlattices for tailored applications in broad-band tunable lasers.
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http://dx.doi.org/10.1021/acsomega.8b02837 | DOI Listing |
J Mech Behav Biomed Mater
December 2024
Trinity Centre for Biomedical Engineering, Trinity Biomedical Sciences Institute, Trinity College Dublin, 2, Dublin, Ireland; Discipline of Mechanical, Manufacturing, and Biomedical Engineering, School of Engineering, Trinity College Dublin, 2, Dublin, Ireland; Advanced Materials and Bioengineering Research Centre (AMBER), Trinity College Dublin, Ireland. Electronic address:
Aortic stenosis is a prevalent disease that is treated with either mechanical or bioprosthetic valve replacement devices. However, these implants can experience problems with either functionality in the case of mechanical valves or long-term durability in the case of bioprosthetic valves. To enhance next generation prosthetic valves, such as biomimetic polymeric valves, an improved understanding of the native aortic valve leaflet structure and mechanical response is required to provide much needed benchmarks for future device development.
View Article and Find Full Text PDFUltrasonics
January 2025
College of Aerospace Engineering, Chongqing University, Chongqing 400044, China. Electronic address:
This study delves into the feasibility of leveraging quasi-static component (QSC) generation during primary Lamb wave propagation to discern subtle alterations in the interfacial properties of a two-layered plate. Unlike the second-harmonic generation of Lamb waves, QSC generation doesn't necessitate precise phase-velocity matching but rather requires an approximate matching of group velocities to ensure the emergence of cumulative growth effects. This unique characteristic empowers the QSC-based nonlinear ultrasonic method to effectively surmount the limitations associated with inherent dispersion and multimode traits of Lamb wave propagation.
View Article and Find Full Text PDFProc Natl Acad Sci U S A
January 2025
Department of Chemistry, University of California, Berkeley, CA 94720.
Combining Deep-UV second harmonic generation spectroscopy with molecular simulations, we confirm and quantify the specific adsorption of guanidinium cations to the air-water interface. Using a Langmuir analysis of measurements at multiple concentrations, we extract the Gibbs free energy of adsorption, finding it larger than typical thermal energies. Molecular simulations clarify the role of polarizability in tuning the thermodynamics of adsorption, and establish the preferential parallel alignment of guanidinium at the air-water interface.
View Article and Find Full Text PDFNanomaterials (Basel)
January 2025
Institute of Information Photonics Technology, School of Physics and Optoelectronics, Faculty of Science, Beijing University of Technology, Beijing 100124, China.
Nonlinear optics, a critical branch of modern optics, presents unique potential in the study of two-dimensional (2D) magnetic materials. These materials, characterized by their ultra-thin geometry, long-range magnetic order, and diverse electronic properties, serve as an exceptional platform for exploring nonlinear optical effects. Under strong light fields, 2D magnetic materials exhibit significant nonlinear optical responses, enabling advancements in novel optoelectronic devices.
View Article and Find Full Text PDFAdv Sci (Weinh)
January 2025
Jožef Stefan Institute, Ljubljana, 1000, Slovenia.
The recent discovery of ferroelectric nematic liquid crystalline phases marks a major breakthrough in soft matter research. An intermediate phase, often observed between the nonpolar and the ferroelectric nematic phase, shows a distinct antiferroelectric response to electric fields. However, its structure and formation mechanisms remain debated, with flexoelectric and electrostatics effects proposed as competing mechanisms.
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