The deficiency of nonlinear-optical (NLO) materials in the IR region inspires strong research interest in this field. Here, SnGaS (), crystallizing in the orthorhombic 2 space group, demonstrates obvious NLO activity, around a maximum of 1.6 times that of AgGaS and a strong laser-induced damage threshold of 9.7 times that of AGS. represents the first NLO-active compound in the MMQ (M = divalent Ca, Sr, Ba, Pb, Sn, and Eu; M = B, Al, Ga, and In; Q = S and Se) family. The NLO performances of are systematically studied experimentally and theoretically.
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