SnSe Nanosheets for Subpicosecond Harmonic Mode-Locked Pulse Generation.

Small

CAS Key Laboratory of Standardization and Measurement for Nanotechnology, CAS Center for Excellence in Nanoscience, National Center for Nanoscience and Technology, Beijing, 100190, P. R. China.

Published: September 2019

AI Article Synopsis

Article Abstract

Tin diselenide (SnSe ) nanosheets as novel 2D layered materials have excellent optical properties with many promising application prospects, such as photoelectric detectors, nonlinear optics, infrared photoelectric devices, and ultrafast photonics. Among them, ultrafast photonics has attracted much attention due to its enormous advantages; for instance, extremely fast pulse, strong peak power, and narrow bandwidth. In this work, SnSe nanosheets are fabricated by using solvothermal treatment, and the characteristics of SnSe are systemically investigated. In addition, the solution of SnSe nanosheets is successfully prepared as a fiber-based saturable absorber by utilizing the evanescent field effect, which can bear a high pump power. 31st-order subpicosecond harmonic mode locking is generated in an Er-doped fiber laser, corresponding to the maximum repetition rate of 257.3 MHz and pulse duration of 887 fs. The results show that SnSe can be used as an excellent nonlinear photonic device in many fields, such as frequency comb, lasers, photodetectors, etc.

Download full-text PDF

Source
http://dx.doi.org/10.1002/smll.201902811DOI Listing

Publication Analysis

Top Keywords

snse nanosheets
16
subpicosecond harmonic
8
ultrafast photonics
8
snse
6
nanosheets subpicosecond
4
harmonic mode-locked
4
mode-locked pulse
4
pulse generation
4
generation tin
4
tin diselenide
4

Similar Publications

Prompting CO Electroreduction to Ethanol by Iron Group Metal Ion Dopants Induced Multi-sites at the Interface of SnSe/SnSe p-n Heterojunction.

Angew Chem Int Ed Engl

January 2025

Key Laboratory of Functional Molecular Solids, Ministry of Education, Anhui Engineering Research Center of Carbon Neutrality, Anhui Key Laboratory of Molecule-Based Materials, College of Chemistry and Materials Science, Anhui Normal University, Wuhu, 241002, P. R. China.

The development of non-copper-based materials for CO electroreduction to ethanol with high selectivity at large current density is highly desirable, but still a great challenge. Herein, we report iron group metal ions of M (M=Fe, Co, or Ni)-doped amorphous/crystalline SnSe/SnSe nanorod/nanosheet hierarchical structures (a/c-SnSe/SnSe) for selective CO electroreduction to ethanol. Iron group metal ions doping induces multiple active sites at the interface of M-doped SnSe/SnSe p-n heterojunction, which strengthens *CO intermediate binding for further C-C coupling to eventual ethanol generation.

View Article and Find Full Text PDF
Article Synopsis
  • A new one-pot heating technique was developed to create core/crown SnSe/SnS nanosheets by adjusting the reactivity of sulfur and selenium precursors.
  • The synthesis involves using SnCl and selenium phosphines to form SnSe nanosheets, with the addition of a reactive S-oleylamine complex to grow SnS crowns.
  • Various microscopy methods confirmed the high crystallinity and structure of the resulting core/crown nanosheets.
View Article and Find Full Text PDF

Boosted Near-Infrared Photothermal Conversion in Rare Earth Ions-Doped 2D SnSe Nanosheets for Solar-Powered Water Evaporation Systems.

Small

December 2024

Key Laboratory of Rare Earth Optoelectronic Materials and Devices of Zhejiang Province, China Jiliang University, Hangzhou, 310018, China.

Solar-powered water evaporation as a clean and abundant renewable energy-efficient desalination technology provides a promising strategy to solve the shortage of freshwater resources. However, the development and application of solar vapor technology are hindered by the relatively low near-infrared photothermal conversion efficiency of existing materials and the lack of effective improvement strategies. In this work, the conductivity characteristics of 2D semiconductors are capitalized on the high visible light absorption and ultra-low thermal.

View Article and Find Full Text PDF

Understanding the dynamic transformation processes of electrocatalysts during electrochemical reactions is crucial for the development of advanced materials for energy conversion and storage, yet it remains a challenge. Herein, we report the real-time monitoring of the dynamic transformation of a series of layered Sn chalcogenides during electrochemical reduction using a plasmonic imaging method. Taking SnSe as an example, we observed a strong firework-like emission diffusing outward from SnSe to the surrounding solution under a negative potential.

View Article and Find Full Text PDF

Reducing defects in the active layer is important for improving the crystalline quality of all-inorganic perovskite solar cells (PSCs). Exploring novel additives is one of the most promising approaches to minimize active layer defects. In this work, two-dimensional (2D) SnSe nanosheets with excellent optoelectronic properties are prepared using an ultrasonic exfoliation method.

View Article and Find Full Text PDF

Want AI Summaries of new PubMed Abstracts delivered to your In-box?

Enter search terms and have AI summaries delivered each week - change queries or unsubscribe any time!