The discovery of topological materials has motivated recent developments to export topological concepts into photonics to make light behave in exotic ways. Here, we predict several unconventional quantum optical phenomena that occur when quantum emitters interact with a topological waveguide quantum electrodynamics bath, namely, the photonic analog of the Su-Schrieffer-Heeger model. When the emitters' frequency lies within the topological bandgap, a chiral bound state emerges, which is located on just one side (right or left) of the emitter. In the presence of several emitters, this bound state mediates topological, tunable interactions between them, which can give rise to exotic many-body phases such as double Néel ordered states. Furthermore, when the emitters' optical transition is resonant with the bands, we find unconventional scattering properties and different super/subradiant states depending on the band topology. Last, we propose several implementations where these phenomena can be observed with state-of-the-art technology.
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http://dx.doi.org/10.1126/sciadv.aaw0297 | DOI Listing |
Chemistry
January 2025
Indian Institute of Science Education and Research (IISER), Chemistry, Dr. Homi Bhabha Road, Pashan, 411008, Pune, INDIA.
Metal-organic frameworks (MOFs) are a fascinating class of structured materials with diverse functionality originating from the distinctive physicochemical properties. This review focuses on the specific chemical design of geometrically frustrated MOFs along with the origin of the intriguing magnetic properties. We have discussed the arrangement of spin centres (metal and ligand) which are responsible for the unusual magnetic phenomena in MOFs.
View Article and Find Full Text PDFChemphyschem
January 2025
University of Minnesota Twin Cities, Chemical Engineering and Materials Science, 421 Washington Avenue SE, 55455, Minneapolis, UNITED STATES OF AMERICA.
Broader adoption of 4D ultrafast electron microscopy (UEM) for the study of chemical, materials, and quantum systems is being driven by development of new instruments as well as continuous improvement and characterization of existing technologies. Perhaps owing to the still-high barrier to entry, the full range of capabilities of laser-driven 4D UEM instruments has yet to be established, particularly when operated at extremely low beam currents (~fA). Accordingly, with an eye on beam stability, we have conducted particle tracing simulations of unconventional off-axis photoemission geometries in a UEM equipped with a thermionic-emission gun.
View Article and Find Full Text PDFJ Colloid Interface Sci
January 2025
Faculty of Science, Kunming University of Science and Technology, Kunming 650500, China.
The fabrication of dual-quantum dot heterostructures offers a promising strategy to enhance the environmental remediation performance of photocatalysts. Herein, a BiWO-based Z-scheme heterojunction was constructed by incorporating carbonized polymer dots (CPDs) and CdS quantum dots (QDs) via a microwave-assisted solvothermal method. The 1 wt% CPDs/CdS QDs/BiWO (CCBW-1) composite achieved optimal Cr(VI) removal, reaching 97.
View Article and Find Full Text PDFACS Nano
January 2025
Department of Physics and Astronomy, Interdisciplinary Nanoscience Center, Aarhus University, Aarhus C 8000, Denmark.
Superlattices from twisted graphene mono- and bilayer systems give rise to on-demand many-body states such as Mott insulators and unconventional superconductors. These phenomena are ascribed to a combination of flat bands and strong Coulomb interactions. However, a comprehensive understanding is lacking because the low-energy band structure strongly changes when an electric field is applied to vary the electron filling.
View Article and Find Full Text PDFMaterials (Basel)
December 2024
Department of Applied Physics, Institute of Natural Sciences, Kyung Hee University, Yongin 17104, Republic of Korea.
SrCu(BO) (Sr-122) has attracted considerable interest as a quasi-two-dimensional S = 1/2 Heisenberg antiferromagnetic spin system with a Shastry-Sutherland lattice (SSL) structure. It features a Cu spin dimer ground state and exhibits intra-dimer Dzyaloshinskii-Moriya interactions, making Sr-122 a fascinating platform for studying quantum magnetic phenomena. In this study, we investigate the β-phase of SrCu(BO) (β-Sr-212), which retains the same spin structure as Sr-122, to explore how the carrier concentration affects the spin gap.
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