We present experimental data and a complete theoretical description of the magneto-optical contributions to the complex refractive index in the extreme ultraviolet (XUV) range covering the 3p resonances of Fe, Co, and Ni. The direct comparison of the two allows us to conclude that many-body corrections to the ground state and local field effects are crucial for an accurate description of M-edge spectra. Our results are relevant for investigation of static magnetization, via XUV spectroscopy of multielement systems, as well as the dynamics of magnetization, as needed in the study of femtomagnetism and spintronics.
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http://dx.doi.org/10.1103/PhysRevLett.122.217202 | DOI Listing |
Adv Sci (Weinh)
January 2025
Technical Center for Multifunctional Magneto-Optical Spectroscopy (Shanghai), Engineering Research Center of Nanophotonics & Advanced Instrument (Ministry of Education), Department of Physics, School of Physics and Electronic Science, East China Normal University, Shanghai, 200241, China.
Controlling polarization states of ferroelectrics can enrich optoelectronic properties and functions, offering a new avenue for designing advanced electronic and optoelectronic devices. Here, ferroelectric semiconductor-based field-effect transistors (FeSFETs) are fabricated, where the channel is a ferroelectric semiconductor (e.g.
View Article and Find Full Text PDFIn this Letter, we calculate the optical and magneto-optical reflectivity in a dielectric/gap/ferromagnet excited by a -polarized monochromatic optical beam through the prism (Otto configuration) as a function of the angle of incidence and the gap thickness . Besides the well-known surface plasmon polariton (SPP resonance at ∼ ), we find a new, to the best of our knowledge, resonance with a nanometric gap ∼ 10 nm at a large ∼ 80°. Both resonances display pronounced resonant behavior in the transverse magneto-optical Kerr effect (T-MOKE).
View Article and Find Full Text PDFNanophotonics
November 2024
Universite Claude Bernard Lyon 1, CNRS, Institut Lumière Matière, UMR5306, F-69100, Villeurbanne, France.
In view of the recent increased interest in light-induced manipulation of magnetism in nanometric length scales this work presents metal clusters as promising elementary units for generating all-optical ultrafast magnetization. We perform a theoretical study of the opto-magnetic properties of metal clusters through ab-initio real-time (RT) simulations in real-space using time-dependent density functional theory (TDDFT). Through ab-initio calculations of plasmon excitation with circularly polarized laser pulse in atomically precise clusters of simple and noble metals, we discuss the generation of orbital magnetic moments due to the transfer of angular momentum from light field through optical absorption at resonance energies.
View Article and Find Full Text PDFRev Sci Instrum
November 2024
National Institute of Chemical Physics and Biophysics, Akadeemia tee 23, 12618 Tallinn, Estonia.
We present a magneto-optical Kerr effect (MOKE) spectrometer based on a modified Martin-Puplett interferometer, utilizing continuous wave sub-THz low-power radiation in a broad frequency range. This spectrometer is capable of measuring the frequency dependence of the MOKE response function, both the Kerr rotation and ellipticity, simultaneously, with accuracy limited by a sub-milliradian threshold, without the need for a reference measurement. The instrument's versatility allows it to be coupled to a cryostat with optical windows, enabling studies of a variety of quantum materials such as unconventional superconductors, two-dimensional electron gas systems, quantum magnets, and other systems showing optical Hall response at sub-Kelvin temperatures and in high magnetic fields.
View Article and Find Full Text PDFPhys Rev E
October 2024
Institut für Physik, Johannes Gutenberg-Universität Mainz, Staudingerweg 7, 55128 Mainz, Germany.
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