We demonstrate the generation of nanosecond mid-infrared pulses via fast modulation of thermal emissivity enabled by the absorption of visible pump pulses in unpatterned silicon and gallium arsenide. The free-carrier dynamics in these materials result in nanosecond-scale modulation of thermal emissivity, which leads to nanosecond pulsed thermal emission. To our knowledge, the nanosecond thermal-emissivity modulation in this work is three orders of magnitude faster than what has been previously demonstrated. We also indirectly observed subnanosecond thermal pulses from hot carriers in semiconductors. The experiments are well described by our multiphysics model. Our method of converting visible pulses into the mid infrared using modulated emissivity obeys different scaling laws and can have significant wavelength tunability compared to approaches based on conventional nonlinearities.
Download full-text PDF |
Source |
---|---|
http://www.ncbi.nlm.nih.gov/pmc/articles/PMC6548774 | PMC |
http://dx.doi.org/10.1038/s41377-019-0158-6 | DOI Listing |
Langmuir
January 2025
Institute of Physics, Czech Academy of Sciences, Na Slovance 2, 182 21 Prague 8, Czech Republic.
Black aluminum is a material characterized by high surface porosity due to columnar growth and exhibits unique optical properties that make it attractive for applications such as light trapping, infrared detection, and passive thermal radiation cooling. In this study, we correlate the structural and optical properties of black aluminum by comparing it with conventional reflective aluminum layers. These layers of varying thicknesses were deposited on fused silica substrates, and their optical properties were analyzed.
View Article and Find Full Text PDFACS Appl Mater Interfaces
January 2025
School of Energy and Environment, City University of Hong Kong, Kowloon 999077, Hong Kong.
Radiative cooling textiles designed to reflect incoming sunlight and enhance mid-infrared (MIR) emissivity show great potential for ensuring personal thermal comfort. Thus, these textiles are gaining prominence as a means of combating the heat stress induced by global warming. Nonetheless, integrating radiative cooling effects into scalable textile materials for personal thermoregulation remains a formidable challenge.
View Article and Find Full Text PDFAdv Mater
December 2024
Key Laboratory of Material Chemistry for Energy Conversion and Storage, Ministry of Education, Hubei Key Laboratory of Material Chemistry and Service Failure and Hubei Engineering Research Center for Biomaterials and Medical Protective Materials, Huazhong University of Science and Technology, Wuhan, 430074, P. R. China.
The development of zero-power moisture-harvesting technology in an unsaturated atmosphere is of great significance for coping with global freshwater scarcity. Here, inspired by Pachydactylus rangei's (Namib sand gecko) ability to evade thermal radiation and harvest moisture, a power-free cooling moisture harvester (PFCMH) is fabricated using the continuous, industrialized micro-extrusion compression molding. A Luneburg lens is introduced in the PFCMH for the first time, endowing it with a high reflectivity of ≈92.
View Article and Find Full Text PDFInt J Biol Macromol
December 2024
Jiangsu Optoelectronic Functional Materials Engineering Research Center, School of Chemistry and Chemical Engineering, Southeast University, Nanjing 211189, China. Electronic address:
Passive radiative cooling (PRC) is an emerging sustainable technology that plays a key role for achieving the goal of carbon neutrality. However, several challenges remain for PRC materials in their practical application in building thermal management, including overcooling problems and unsatisfactory cooling efficiency caused by solar absorption and parasitic heat gains. In this work, fluorinated cellulose-based composite aerogels (FCCA) integrating thermal insulation and PRC were developed by a facile manufacturing strategy that combined phase separation and freeze-drying.
View Article and Find Full Text PDFNanomicro Lett
December 2024
Jiangsu Key Laboratory of Electrochemical Energy Storage Technologies, College of Materials Science and Technology, Nanjing University of Aeronautics and Astronautics, Nanjing, 210016, People's Republic of China.
Dual-band electrochromic devices capable of the spectral-selective modulation of visible (VIS) light and near-infrared (NIR) can notably reduce the energy consumption of buildings and improve the occupants' visual and thermal comfort. However, the low optical modulation and poor durability of these devices severely limit its practical applications. Herein, we demonstrate an efficient and flexible bifunctional dual-band electrochromic device which not only shows excellent spectral-selective electrochromic performance with a high optical modulation and a long cycle life, but also displays a high capacitance and a high energy recycling efficiency of 51.
View Article and Find Full Text PDFEnter search terms and have AI summaries delivered each week - change queries or unsubscribe any time!