X-ray Thomson scattering experiments in the soft and hard x-ray regime yield information on fundamental parameters of high-density systems. Pump-probe experiments with variable time delay provide insight into the excitation and relaxation dynamics in dense plasmas. On short time scales, a local thermodynamic equilibrium description might not be sufficient. Besides nonequilibrium effects on the electron distribution function, spatial inhomogeneities influence the scattering signal. Generalizing previous approaches of Belyi [Phys. Rev. E 97, 053204 (2018)2470-004510.1103/PhysRevE.97.053204] and Kozlowski et al. [Sci. Rep. 6, 24283 (2016)2045-232210.1038/srep24283], we discuss implications for Thomson scattering spectra for inhomogeneous plasmas in the warm dense matter regime based on a gradient expansion within real-time Green's-functions theory. Especially in the collective scattering regime, Thomson scattering spectra are modifed substantially by spatial inhomogeneities. Within a first-order gradient expansion, the dispersion relation for plasmons is determined. In particular, the ratio of the heights of the plasmon peaks is changed which prevents a simple estimation of the plasma temperature from the detailed balance relation.
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http://dx.doi.org/10.1103/PhysRevE.99.053205 | DOI Listing |
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