AI Article Synopsis

  • The study examines various magnetic properties of the Kitaev honeycomb iridate Cu2IrO3, revealing that even with chemical disorders, there are no signs of spin glass behavior down to 260 mK.
  • Despite the lack of static magnetism, the results indicate dynamic spin behavior, as shown by muon spin relaxation measurements.
  • Scaling relations in magnetic susceptibility and magnetization suggest the influence of bond randomness, but specific heat measurements point to unexpected low-lying excitations, highlighting the complex effects of quenched disorder in this spin system.

Article Abstract

We report on magnetization M(H), dc and ac magnetic susceptibility χ(T), specific heat C_{m}(T) and muon spin relaxation (μSR) measurements of the Kitaev honeycomb iridate Cu_{2}IrO_{3} with quenched disorder. In spite of the chemical disorders, we find no indication of spin glass down to 260 mK from the C_{m}(T) and μSR data. Furthermore, a persistent spin dynamics observed by the zero-field muon spin relaxation evidences an absence of static magnetism. The remarkable observation is a scaling relation of χ[H,T] and M[H,T] in H/T with the scaling exponent α=0.26-0.28, expected from bond randomness. However, C_{m}[H,T]/T disobeys the predicted universal scaling law, pointing towards the presence of additional low-lying excitations on the background of bond-disordered spin liquid. Our results signify a many-faceted impact of quenched disorder in a Kitaev spin system due to its peculiar bond character.

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http://dx.doi.org/10.1103/PhysRevLett.122.167202DOI Listing

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