Air pollution can cause acute and chronic health problems. It has many components, and one component of interest is volatile organic compounds (VOCs). While the outdoor environment may have regulations regarding exposure limits, the indoor environment is often unregulated and VOCs often appear in greater concentrations in the indoor environment. Therefore, it is equally critical to monitor both the indoor and outdoor environments for ambient chemical levels that an individual person is exposed to. While a number of different chemical detectors exist, most lack the ability to provide portable monitoring. We have developed a portable and wearable sampler that collects environmental VOCs in a person's immediate "exposure envelope" onto custom micro-preconcentrator chips for later benchtop analysis. The system also records ambient temperature and humidity and the GPS location during sampling, and the chip cartridges can be used in sequence over time to complete a profile of individual chemical exposure over the course of hours/days/weeks/months. The system can be programmed to accumulate sample for various times with varying periodicity. We first tested our sampler in the laboratory by completing calibration curves and testing saturation times for various common chemicals. The sampler was also tested in the field by collecting both indoor and outdoor personal exposure samples. Additionally under IRB approval, a teenaged volunteer wore the sampler for 5 days during which it sampled periodically throughout a 12 h period each day and the volunteer replaced the micro-preconcentrator chip each day.
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http://dx.doi.org/10.1021/acssensors.9b00304 | DOI Listing |
J Food Sci
January 2025
Digital Agriculture, Food and Wine Research Group, School of Agriculture, Food and Ecosystem Science, Faculty of Science, The University of Melbourne, Melbourne, Victoria, Australia.
Fraud in alcoholic beverages through counterfeiting and adulteration is rising, significantly impacting companies economically. This study aimed to develop a method using near-infrared (NIR) spectroscopy (1596-2396 nm) through the bottle, along with machine learning (ML) modeling for beer authentication, quality traits, and control assessment. For this study, 25 commercial beers from different brands, styles, and three types of fermentation were used.
View Article and Find Full Text PDFMetabolomics
January 2025
Owlstone Medical Ltd., Cambridge, UK.
Introduction: Breath Volatile organic compounds (VOCs) are promising biomarkers for clinical purposes due to their unique properties. Translation of VOC biomarkers into the clinic depends on identification and validation: a challenge requiring collaboration, well-established protocols, and cross-comparison of data. Previously, we developed a breath collection and analysis method, resulting in 148 breath-borne VOCs identified.
View Article and Find Full Text PDFAnal Methods
January 2025
Marine Elements and Marine Environment Division, CSIR-Central Salt & Marine Chemicals Research Institute, Bhavnagar 364 002, Gujarat, India.
Monitoring persistent organic pollutants (POPs) with endocrine-disrupting properties poses significant analytical challenges due to labor-intensive, costly, and environmentally unsustainable procedures. This study developed an efficient and robust approach for the simultaneous detection of diverse groups of semi-volatile organics in water and sediment samples using gas chromatography-tandem mass spectrometry (GC-MS). Two extraction methods were studied for determining POPs in water and sediments.
View Article and Find Full Text PDFPNAS Nexus
January 2025
Thrust of Earth, Ocean and Atmospheric Sciences Function Hub, The Hong Kong University of Science and Technology (Guangzhou), Guangzhou 511453, China.
Modulating the electronic structure of noble metals via electronic metal-support interaction (EMSI) has been proven effectively for facilitating molecular oxygen activation and catalytic oxidation reactions. Nevertheless, the investigation of the fundamental mechanisms underlying activity enhancement has primarily focused on metal oxides as supports, especially in the catalytic degradation of volatile organic compounds. In this study, a novel Pt catalyst supported on nitrogen-doped carbon encapsulating FeNi alloy, featuring ultrafine Pt nanoparticles, was synthesized.
View Article and Find Full Text PDFFood Chem X
January 2025
Spice and Beverage Research Institute, Chinese Academy of Tropical Agricultural Sciences/ Hainan Provincial Key Laboratory of Genetic Improvement and Quality Regulation for Tropical Spice and Beverage Crops/ Key Laboratory of Genetic Resource Utilization of Spice and Beverage Crops, Ministry of Agriculture and Rural Affairs, Wanning, Hainan 571533, China.
Pandan ( Roxb.) are one of the traditional food materials in Southeast Asian countries. However, there has long been a lack of understanding of the differences in volatile organic compounds (VOCs) of leaves at different growth periods.
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